Vincent Wanie, Pasquale Barbato, Josina Hahne, Sergey Ryabchuk, Ammar Bin Wahid, David Amorim, Erik P Månsson, Andrea Trabattoni, Roberto Osellame, Rebeca Martínez Vázquez, Francesca Calegari
{"title":"Ultraviolet supercontinuum generation using a differentially-pumped integrated glass chip","authors":"Vincent Wanie, Pasquale Barbato, Josina Hahne, Sergey Ryabchuk, Ammar Bin Wahid, David Amorim, Erik P Månsson, Andrea Trabattoni, Roberto Osellame, Rebeca Martínez Vázquez, Francesca Calegari","doi":"10.1088/2515-7647/ad2bd3","DOIUrl":null,"url":null,"abstract":"We investigate the generation of ultrabroadband femtosecond ultraviolet (UV) radiation via third-order harmonic generation in highly confined gas media. A dual-stage differential-pumping scheme integrated into a glass microfluidic chip provides an exceptional gas confinement up to several bar and allows the apparatus to be operated under high-vacuum environment. UV pulses are generated both in argon and neon with up to ∼0.8 <italic toggle=\"yes\">μ</italic>J energy and 0.2% conversion efficiency for spectra that cover the UVB and UVC regions between 200 and 325 nm. Numerical simulations based on the unidirectional pulse propagation equation reveal that ionization plays a critical role for extending the spectral bandwidth of the generated third-harmonic pulse beyond the tripled 800 nm driving laser pulse bandwidth. By delivering UV supercontinua supporting Fourier transform limits below 2 fs, as well as comparable pulse energies with respect to capillary-based techniques that typically provide high spectral tunability but produce narrower bandwidths, our compact device makes a step forward towards the production and application of sub-fs UV pulses for the investigation of electron dynamics in neutral molecules.","PeriodicalId":44008,"journal":{"name":"Journal of Physics-Photonics","volume":null,"pages":null},"PeriodicalIF":4.6000,"publicationDate":"2024-03-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Physics-Photonics","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1088/2515-7647/ad2bd3","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"OPTICS","Score":null,"Total":0}
引用次数: 0
Abstract
We investigate the generation of ultrabroadband femtosecond ultraviolet (UV) radiation via third-order harmonic generation in highly confined gas media. A dual-stage differential-pumping scheme integrated into a glass microfluidic chip provides an exceptional gas confinement up to several bar and allows the apparatus to be operated under high-vacuum environment. UV pulses are generated both in argon and neon with up to ∼0.8 μJ energy and 0.2% conversion efficiency for spectra that cover the UVB and UVC regions between 200 and 325 nm. Numerical simulations based on the unidirectional pulse propagation equation reveal that ionization plays a critical role for extending the spectral bandwidth of the generated third-harmonic pulse beyond the tripled 800 nm driving laser pulse bandwidth. By delivering UV supercontinua supporting Fourier transform limits below 2 fs, as well as comparable pulse energies with respect to capillary-based techniques that typically provide high spectral tunability but produce narrower bandwidths, our compact device makes a step forward towards the production and application of sub-fs UV pulses for the investigation of electron dynamics in neutral molecules.