Correlations in strong-field-emitted ultrashort electron pulses from metal needle tips

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-02-29 DOI:10.1088/1612-202x/ad2b5a
S Meier, J Heimerl, P Hommelhoff
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Abstract

When two electrons are emitted from a metal needle tip with the help of femtosecond laser pulses, they show a strong anticorrelation signal in the energy domain. Depending on the wavelength and intensity of the driving laser pulses, the electron emission process can be either in a perturbative regime, like single- or multi-photon photoemission, or in the strong-field regime, where emission is dominated by the instantaneous electric field of the laser pulse, or in the intermediate regime. Here, we report on the two-electron anticorrelation signal and how it evolves from the multiphoton toward the strong-field emission regime. We show that in both cases, the resulting anticorrelation signal can be well explained by semi-classical simulations using a point-particle model, thus the dynamics is dominated by the center-of-mass dynamics of the individual electrons. However, the actual emission process of multiple interacting electrons requires improved quantum mechanical models and therefore remains the subject of future work.This paper is part of the Special Topic Collection: papers from the 31th Annual International Laser Physics Workshop 2023 (LPHYS 2023).
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金属针尖强场发射超短电子脉冲的相关性
当两个电子在飞秒激光脉冲的帮助下从金属针尖发射出来时,它们在能域中显示出强烈的反相关信号。根据驱动激光脉冲的波长和强度,电子发射过程既可以处于扰动状态(如单光子或多光子光电子发射),也可以处于强场状态(发射由激光脉冲的瞬时电场主导),还可以处于中间状态。在此,我们报告了双电子反相关信号及其如何从多光子向强场发射机制演变。我们的研究表明,在这两种情况下,所产生的反相关信号都能通过使用点粒子模型的半经典模拟得到很好的解释,因此其动力学是由单个电子的质量中心动力学所主导的。然而,多个相互作用电子的实际发射过程需要改进的量子力学模型,因此仍是未来工作的主题。本文是 "专题文集:第 31 届 2023 国际激光物理研讨会(LPHYS 2023)论文 "的一部分。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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