Characterizing PFAS concentrations in drinking water treatment residuals

Conner C. Murray, Alexander S. Gorzalski, Erik J. Rosenfeldt, Christine Owen, Chris Moody
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Abstract

While drinking water treatment plants (DWTPs) are not considered a source of per- and polyfluoroalkyl substances (PFAS), PFAS concentrate in treatment residuals relative to their source water concentrations. Regulatory actions considered for PFAS-impacted residuals could affect the cost and viability of conventional residual management practices. This study estimated the annual quantity of residuals generated in the United States and presents a framework for understanding how PFAS may concentrate in these residual streams. Findings of this work indicate that PFAS may substantially impact DWTP residuals management, especially coagulation and softening solids, at concentration factors greater than 100 and spent adsorbents at PFAS concentration factors greater than 10,000. If potential regulatory actions were to apply to coagulation and softening residuals, those regulations must consider impacts on disposal of more than 420,000,000 wet tons of at-risk DWTP residuals which are generated annually.

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确定饮用水处理残留物中 PFAS 的浓度特征
虽然饮用水处理厂 (DWTP) 不被视为全氟烷基和多氟烷基物质 (PFAS) 的来源,但相对于原水浓度而言,PFAS 会在处理残留物中富集。针对受 PFAS 影响的残留物而考虑采取的监管措施可能会影响传统残留物管理方法的成本和可行性。这项研究估算了美国每年产生的残留物数量,并提出了一个框架,用于了解 PFAS 如何在这些残留物流中富集。研究结果表明,当 PFAS 浓度系数大于 100 时,PFAS 可能会对污水处理厂的残留物管理产生重大影响,尤其是混凝和软化固体,而当 PFAS 浓度系数大于 10,000 时,则会对废吸附剂产生重大影响。如果要对混凝和软化残留物采取潜在的监管措施,这些法规必须考虑对每年产生的超过 4.2 亿湿吨高风险 DWTP 残留物处置的影响。
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