Advancements on metal oxide semiconductor photocatalysts in photo-electrochemical conversion of carbon dioxide into fuels and other useful products

IF 3.1 4区 工程技术 Q3 ENERGY & FUELS Frontiers in Energy Pub Date : 2024-03-20 DOI:10.1007/s11708-024-0939-3
Jai Prakash, Zhangsen Chen, Shakshi Saini, Gaixia Zhang, Shuhui Sun
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Abstract

Due to its fascinating and tunable optoelectronic properties, semiconductor nanomaterials are the best choices for multidisciplinary applications. Particularly, the use of semiconductor photocatalysts is one of the promising ways to harness solar energy for useful applications in the field of energy and environment. In recent years, metal oxide-based tailored semiconductor photocatalysts have extensively been used for photocatalytic conversion of carbon dioxide (CO2) into fuels and other useful products utilizing solar energy. This is very significant not only from renewable energy consumption but also from reducing global warming point of view. Such current research activities are promising for a better future of society. The present mini-review is focused on recent developments (2–3 years) in metal oxide semiconductor hybrid photocatalysts-based photo-electrochemical conversion of CO2 into fuels and other useful products. First, general mechanism of photo-electrochemical conversion of CO2 into fuels or other useful products has been discussed. Then, various metal oxide-based emerging hybrid photocatalysts including tailoring of their morphological, compositional, and optoelectronic properties have been discussed with emphasis on their role in enhancing photo-electrochemical efficienty. Afterwards, mechanism of their photo-electrochemical reactions and applications in CO2 conversion into fuels/other useful products have been discussed. Finally, challenges and future prospects have been discussed followed by a summary.

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金属氧化物半导体光催化剂在光电化学将二氧化碳转化为燃料和其他有用产品方面的进展
半导体纳米材料具有迷人的可调光电特性,是多学科应用的最佳选择。特别是,使用半导体光催化剂是利用太阳能在能源和环境领域进行有用应用的一种前景广阔的方法。近年来,基于金属氧化物的定制半导体光催化剂已被广泛用于利用太阳能将二氧化碳(CO2)光催化转化为燃料和其他有用产品。这不仅从可再生能源消费的角度,而且从减少全球变暖的角度来看,都具有非常重要的意义。目前的这些研究活动有望为社会带来更美好的未来。本微型综述侧重于基于金属氧化物半导体混合光催化剂的光电化学将二氧化碳转化为燃料和其他有用产品的最新进展(2-3 年)。首先,讨论了光电化学将二氧化碳转化为燃料或其他有用产品的一般机理。然后,讨论了各种基于金属氧化物的新兴混合光催化剂,包括调整其形态、组成和光电特性,重点是它们在提高光电化学效率方面的作用。随后,讨论了它们的光电化学反应机理以及在将二氧化碳转化为燃料/其他有用产品方面的应用。最后,讨论了挑战和未来前景,并进行了总结。
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来源期刊
Frontiers in Energy
Frontiers in Energy Energy-Energy Engineering and Power Technology
CiteScore
5.90
自引率
6.90%
发文量
708
期刊介绍: Frontiers in Energy, an interdisciplinary and peer-reviewed international journal launched in January 2007, seeks to provide a rapid and unique platform for reporting the most advanced research on energy technology and strategic thinking in order to promote timely communication between researchers, scientists, engineers, and policy makers in the field of energy. Frontiers in Energy aims to be a leading peer-reviewed platform and an authoritative source of information for analyses, reviews and evaluations in energy engineering and research, with a strong focus on energy analysis, energy modelling and prediction, integrated energy systems, energy conversion and conservation, energy planning and energy on economic and policy issues. Frontiers in Energy publishes state-of-the-art review articles, original research papers and short communications by individual researchers or research groups. It is strictly peer-reviewed and accepts only original submissions in English. The scope of the journal is broad and covers all latest focus in current energy research. High-quality papers are solicited in, but are not limited to the following areas: -Fundamental energy science -Energy technology, including energy generation, conversion, storage, renewables, transport, urban design and building efficiency -Energy and the environment, including pollution control, energy efficiency and climate change -Energy economics, strategy and policy -Emerging energy issue
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