The Source of Parabens in Urban River Water: The Evidence From Outdoor Multimedia Environment in Six Metropolitan Cities, China

IF 8.9 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Environmental Science & Technology Letters Environ. Pub Date : 2024-04-12 DOI:10.1021/acs.estlett.4c00213
Xue Zhao, Yawei Wang*, Zhigang Li and Tianyu Chen, 
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Abstract

Parabens (PBs) are typical endocrine disrupting compounds (EDCs) that are commonly found in a water environment. However, their fate and transport in urban rivers remain largely unexplored. This study offers a quantitative analysis of the sources of PBs in urban river water, considering the perspective of a multimedia environment. PBs were ubiquitous in the surface water of six metropolitan cities in China, with median concentrations of 8.38 ng/L. A significant difference was observed for PB concentrations in different cities. The geographical variation of PBs in the six rivers may be influenced by multiple factors, including hydrological conditions (runoff amounts and catchment areas), environmental factors (temperature and SPM concentrations), population density, production, and domestic wastewater discharge. Here, the occurrence of PBs in outdoor dust was reported for the first time and was found to be the most polluted solid medium on the land surface. The estimated input fluxes of PBs in the six rivers ranged from 32.0 to 1470 tons/a. The point source emission was the primary input source of PBs in river water of the six cities, contributing between 56.7% and 93.7%, followed by the non-point source discharge of runoff scouring dust, contributing 1.77% to 38.4%.

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城市河水中对羟基苯甲酸酯的来源:来自中国六个大都市室外多媒体环境的证据
对羟基苯甲酸酯(PBs)是水环境中常见的典型内分泌干扰化合物(EDCs)。然而,它们在城市河流中的归宿和迁移在很大程度上仍未得到研究。本研究从多媒体环境的角度出发,对城市河水中 PBs 的来源进行了定量分析。在中国六个大城市的地表水中,多溴联苯无处不在,浓度中位数为 8.38 纳克/升。不同城市的 PB 浓度存在明显差异。六条河流中 PBs 的地域差异可能受到多种因素的影响,包括水文条件(径流量和集水区)、环境因素(温度和 SPM 浓度)、人口密度、生产和生活污水排放。本文首次报道了室外灰尘中出现的多溴联苯,并发现多溴联苯是陆地表面污染最严重的固体介质。六条河流中的多溴联苯估计输入通量从 32.0 吨/a 到 1470 吨/a 不等。点源排放是六个城市河水中多溴联苯的主要输入源,占 56.7% 至 93.7%,其次是径流冲刷尘的非点源排放,占 1.77% 至 38.4%。
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来源期刊
Environmental Science & Technology Letters Environ.
Environmental Science & Technology Letters Environ. ENGINEERING, ENVIRONMENTALENVIRONMENTAL SC-ENVIRONMENTAL SCIENCES
CiteScore
17.90
自引率
3.70%
发文量
163
期刊介绍: Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.
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