Highly efficient three-dimensional solar evaporator for zero liquid discharge desalination of high-salinity brine

IF 19.5 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Carbon Energy Pub Date : 2024-04-05 DOI:10.1002/cey2.548
Meichun Ding, Demin Zhao, Panpan Feng, Baolei Wang, Zhenying Duan, Rui Wei, Yuxi Zhao, Chen-Yang Liu, Chenwei Li
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Abstract

Solar-driven interfacial evaporation is a promising technology for freshwater production from seawater, but salt accumulation on the evaporator surface hinders its performance and sustainability. In this study, we report a simple and green strategy to fabricate a three-dimensional porous graphene spiral roll (3GSR) that enables highly efficient solar evaporation, salt collection, and water production from near-saturated brine with zero liquid discharge (ZLD). The 3GSR design facilitates energy recovery, radial brine transport, and directional salt crystallization, thereby resulting in an ultrahigh evaporation rate of 9.05 kg m−2 h−1 in 25 wt% brine under 1-sun illumination for 48 h continuously. Remarkably, the directional salt crystallization on its outer surface not only enlarges the evaporation area but also achieves an ultrahigh salt collection rate of 2.92 kg m−2 h−1, thus enabling ZLD desalination. Additionally,  3GSR exhibits a record-high water production rate of 3.14 kg m−2 h−1 in an outdoor test. This innovative solution offers a highly efficient and continuous solar desalination method for water production and ZLD brine treatment, which has great implications for addressing global water scarcity and environmental issues arising from brine disposal.

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用于高盐度盐水零排放脱盐的高效三维太阳能蒸发器
太阳能驱动的界面蒸发是从海水中生产淡水的一项前景广阔的技术,但蒸发器表面的盐分积累阻碍了其性能和可持续性。在本研究中,我们报告了一种制造三维多孔石墨烯螺旋辊(3GSR)的简单而绿色的策略,这种辊可实现高效的太阳能蒸发、盐分收集以及从零液体排放(ZLD)的近饱和盐水中生产水。3GSR 的设计有利于能量回收、盐水径向输送和盐的定向结晶,从而使 25 wt% 的盐水在 1 太阳光照射下连续 48 小时的超高蒸发率达到 9.05 kg m-2 h-1。值得注意的是,其外表面的定向盐结晶不仅扩大了蒸发面积,还实现了 2.92 kg m-2 h-1 的超高盐收集率,从而实现了 ZLD 海水淡化。此外,在室外测试中,3GSR 的产水率达到了创纪录的 3.14 kg m-2 h-1。这一创新解决方案提供了一种高效、连续的太阳能海水淡化方法,可用于制水和 ZLD 盐水处理,对解决全球水资源短缺和盐水处理引起的环境问题具有重大意义。
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来源期刊
Carbon Energy
Carbon Energy Multiple-
CiteScore
25.70
自引率
10.70%
发文量
116
审稿时长
4 weeks
期刊介绍: Carbon Energy is an international journal that focuses on cutting-edge energy technology involving carbon utilization and carbon emission control. It provides a platform for researchers to communicate their findings and critical opinions and aims to bring together the communities of advanced material and energy. The journal covers a broad range of energy technologies, including energy storage, photocatalysis, electrocatalysis, photoelectrocatalysis, and thermocatalysis. It covers all forms of energy, from conventional electric and thermal energy to those that catalyze chemical and biological transformations. Additionally, Carbon Energy promotes new technologies for controlling carbon emissions and the green production of carbon materials. The journal welcomes innovative interdisciplinary research with wide impact. It is indexed in various databases, including Advanced Technologies & Aerospace Collection/Database, Biological Science Collection/Database, CAS, DOAJ, Environmental Science Collection/Database, Web of Science and Technology Collection.
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Issue Information Cover Image, Volume 6, Number 10, October 2024 Back Cover Image, Volume 6, Number 10, October 2024 Interface and doping engineering of V2C-MXene-based electrocatalysts for enhanced electrocatalysis of overall water splitting Issue Information
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