Highly efficient three-dimensional solar evaporator for zero liquid discharge desalination of high-salinity brine

IF 19.5 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Carbon Energy Pub Date : 2024-04-05 DOI:10.1002/cey2.548
Meichun Ding, Demin Zhao, Panpan Feng, Baolei Wang, Zhenying Duan, Rui Wei, Yuxi Zhao, Chen-Yang Liu, Chenwei Li
{"title":"Highly efficient three-dimensional solar evaporator for zero liquid discharge desalination of high-salinity brine","authors":"Meichun Ding,&nbsp;Demin Zhao,&nbsp;Panpan Feng,&nbsp;Baolei Wang,&nbsp;Zhenying Duan,&nbsp;Rui Wei,&nbsp;Yuxi Zhao,&nbsp;Chen-Yang Liu,&nbsp;Chenwei Li","doi":"10.1002/cey2.548","DOIUrl":null,"url":null,"abstract":"<p>Solar-driven interfacial evaporation is a promising technology for freshwater production from seawater, but salt accumulation on the evaporator surface hinders its performance and sustainability. In this study, we report a simple and green strategy to fabricate a three-dimensional porous graphene spiral roll (3GSR) that enables highly efficient solar evaporation, salt collection, and water production from near-saturated brine with zero liquid discharge (ZLD). The 3GSR design facilitates energy recovery, radial brine transport, and directional salt crystallization, thereby resulting in an ultrahigh evaporation rate of 9.05 kg m<sup>−2</sup> h<sup>−1</sup> in 25 wt% brine under 1-sun illumination for 48 h continuously. Remarkably, the directional salt crystallization on its outer surface not only enlarges the evaporation area but also achieves an ultrahigh salt collection rate of 2.92 kg m<sup>−2</sup> h<sup>−1</sup>, thus enabling ZLD desalination. Additionally,  3GSR exhibits a record-high water production rate of 3.14 kg m<sup>−2</sup> h<sup>−1</sup> in an outdoor test. This innovative solution offers a highly efficient and continuous solar desalination method for water production and ZLD brine treatment, which has great implications for addressing global water scarcity and environmental issues arising from brine disposal.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":null,"pages":null},"PeriodicalIF":19.5000,"publicationDate":"2024-04-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.548","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Carbon Energy","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/cey2.548","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

Abstract

Solar-driven interfacial evaporation is a promising technology for freshwater production from seawater, but salt accumulation on the evaporator surface hinders its performance and sustainability. In this study, we report a simple and green strategy to fabricate a three-dimensional porous graphene spiral roll (3GSR) that enables highly efficient solar evaporation, salt collection, and water production from near-saturated brine with zero liquid discharge (ZLD). The 3GSR design facilitates energy recovery, radial brine transport, and directional salt crystallization, thereby resulting in an ultrahigh evaporation rate of 9.05 kg m−2 h−1 in 25 wt% brine under 1-sun illumination for 48 h continuously. Remarkably, the directional salt crystallization on its outer surface not only enlarges the evaporation area but also achieves an ultrahigh salt collection rate of 2.92 kg m−2 h−1, thus enabling ZLD desalination. Additionally,  3GSR exhibits a record-high water production rate of 3.14 kg m−2 h−1 in an outdoor test. This innovative solution offers a highly efficient and continuous solar desalination method for water production and ZLD brine treatment, which has great implications for addressing global water scarcity and environmental issues arising from brine disposal.

Abstract Image

Abstract Image

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
用于高盐度盐水零排放脱盐的高效三维太阳能蒸发器
太阳能驱动的界面蒸发是从海水中生产淡水的一项前景广阔的技术,但蒸发器表面的盐分积累阻碍了其性能和可持续性。在本研究中,我们报告了一种制造三维多孔石墨烯螺旋辊(3GSR)的简单而绿色的策略,这种辊可实现高效的太阳能蒸发、盐分收集以及从零液体排放(ZLD)的近饱和盐水中生产水。3GSR 的设计有利于能量回收、盐水径向输送和盐的定向结晶,从而使 25 wt% 的盐水在 1 太阳光照射下连续 48 小时的超高蒸发率达到 9.05 kg m-2 h-1。值得注意的是,其外表面的定向盐结晶不仅扩大了蒸发面积,还实现了 2.92 kg m-2 h-1 的超高盐收集率,从而实现了 ZLD 海水淡化。此外,在室外测试中,3GSR 的产水率达到了创纪录的 3.14 kg m-2 h-1。这一创新解决方案提供了一种高效、连续的太阳能海水淡化方法,可用于制水和 ZLD 盐水处理,对解决全球水资源短缺和盐水处理引起的环境问题具有重大意义。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
Carbon Energy
Carbon Energy Multiple-
CiteScore
25.70
自引率
10.70%
发文量
116
审稿时长
4 weeks
期刊介绍: Carbon Energy is an international journal that focuses on cutting-edge energy technology involving carbon utilization and carbon emission control. It provides a platform for researchers to communicate their findings and critical opinions and aims to bring together the communities of advanced material and energy. The journal covers a broad range of energy technologies, including energy storage, photocatalysis, electrocatalysis, photoelectrocatalysis, and thermocatalysis. It covers all forms of energy, from conventional electric and thermal energy to those that catalyze chemical and biological transformations. Additionally, Carbon Energy promotes new technologies for controlling carbon emissions and the green production of carbon materials. The journal welcomes innovative interdisciplinary research with wide impact. It is indexed in various databases, including Advanced Technologies & Aerospace Collection/Database, Biological Science Collection/Database, CAS, DOAJ, Environmental Science Collection/Database, Web of Science and Technology Collection.
期刊最新文献
Issue Information Cover Image, Volume 6, Number 10, October 2024 Back Cover Image, Volume 6, Number 10, October 2024 Interface and doping engineering of V2C-MXene-based electrocatalysts for enhanced electrocatalysis of overall water splitting Issue Information
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1