Synergistic effect of porous structure and gradient structure in carbon foam to boost terahertz absorption

IF 8.4 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Journal of Materiomics Pub Date : 2024-04-16 DOI:10.1016/j.jmat.2024.03.008
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Abstract

Creating porous structures and gradient structures are two commonly used design strategies for terahertz (THz) absorption enhancement. However, the synergistic effect of porous structure and gradient structure on THz absorption still remains less explored. Here, we took an almost non-conductive porous carbon foam as raw material, and fabricated an integrated gradient porous carbon foam (PCF) by microwave selective sintering. The experimental results show that the synergistic effect of the porous and gradient structures resulted in a 140% improvement in THz absorption performance. Specifically, an excellent average absorption intensity of −38.8 dB (absorptivity is about 99.99%) is obtained in the frequency range from 0.5 to 4.0 THz. COMSOL simulation and transmission line model were applied to explore the formation mechanism and the gradient loss capabilities of gradient structure. This work not only reveals the synergistic enhancement mechanism of porous and gradient structures for the THz absorption, but also provides new insights into the design of high-performance THz absorbers in the future.

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泡沫碳中多孔结构和梯度结构对促进太赫兹吸收的协同效应
创建多孔结构和梯度结构是太赫兹(THz)吸收增强的两种常用设计策略。然而,关于多孔结构和梯度结构对太赫兹吸收的协同效应的探索仍然较少。在此,我们以一种几乎不导电的多孔泡沫碳为原料,通过微波选择性烧结技术制备了一种集成梯度多孔泡沫碳(PCF)。实验结果表明,在多孔结构和梯度结构的协同作用下,太赫兹吸收性能提高了 140%。具体来说,在 0.5 至 4.0 太赫兹的频率范围内,平均吸收强度达到了出色的 -38.8 dB(吸收率约为 99.99%)。研究人员应用 COMSOL 仿真和传输线模型探索了梯度结构的形成机理和梯度损耗能力。这项工作不仅揭示了多孔结构和梯度结构对太赫兹吸收的协同增强机制,还为未来高性能太赫兹吸收体的设计提供了新的启示。
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来源期刊
Journal of Materiomics
Journal of Materiomics Materials Science-Metals and Alloys
CiteScore
14.30
自引率
6.40%
发文量
331
审稿时长
37 days
期刊介绍: The Journal of Materiomics is a peer-reviewed open-access journal that aims to serve as a forum for the continuous dissemination of research within the field of materials science. It particularly emphasizes systematic studies on the relationships between composition, processing, structure, property, and performance of advanced materials. The journal is supported by the Chinese Ceramic Society and is indexed in SCIE and Scopus. It is commonly referred to as J Materiomics.
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