Multi‐scale study of fluidized bed‐chemical vapour deposition process in nuclear fuel coated particle fabrication for high‐temperature gas‐cooled reactor: A review

Zefan Yan, Lin Jiang, Yu Tian, Rongzheng Liu, Youlin Shao, Bing Liu, Malin Liu
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Abstract

Fluidized bed‐chemical vapour deposition (FB‐CVD) is a kind of key technology used widely in many application fields, such as semiconductors, nuclear energy, energy storage, and catalysts. In recent years, it has drawn much attention in the preparation of nuclear fuel coated particles (CP). It also has long played a crucial role in the preparation of high‐temperature gas‐cooled reactor (HTGR) fuel pebbles. The multi‐scale study of FB‐CVD technology has paid attention to the industrial fabrication of nuclear fuel particles at a large scale. In this paper, the recent FB‐CVD studies of different application fields are summarized first. Then, the recent works of our group in the field of FB‐CVD process in nuclear fuel particle fabrication are summarized. The FB‐CVD process in nuclear fuel particle fabrication and the multi‐scale study of the FB‐CVD process are overviewed in detail. Molecular dynamics (MD) simulation is used to study the CVD process of preparing the coating layer at the micro‐scale. Computational fluid dynamics–discrete element model (CFD‐DEM) simulation is used to study the high‐density particle fluidization, mixing particle fluidization, and particle coating process at the particle scale. Process simulation is used to study the entire FB‐CVD production line at the macro scale. Finally, the great application potential of the multi‐scale coupling study of the FB‐CVD process in the industrial fabrication of nuclear fuel particles is revealed. This paper is helpful to develop the academic research field of fluidized beds. It also has inspiration and reference significance for the expansion of other industrial applications of FB‐CVD.
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流化床-化学气相沉积工艺在高温气冷堆核燃料涂层颗粒制造中的多尺度研究:综述
流化床-化学气相沉积(FB-CVD)是一种广泛应用于半导体、核能、储能、催化剂等众多领域的关键技术。近年来,它在核燃料涂层粒子(CP)的制备中备受关注。长期以来,它在高温气冷堆(HTGR)燃料鹅卵石的制备中也发挥着至关重要的作用。对 FB-CVD 技术的多尺度研究已经关注到核燃料颗粒的大规模工业化制备。本文首先总结了近期不同应用领域的 FB-CVD 研究。然后,总结了我们课题组近期在核燃料颗粒制造中的 FB-CVD 工艺领域所做的工作。详细介绍了核燃料颗粒制造中的 FB-CVD 过程以及 FB-CVD 过程的多尺度研究。分子动力学(MD)模拟用于研究微观尺度上制备涂层的 CVD 过程。计算流体动力学-离散元模型(CFD-DEM)模拟用于研究颗粒尺度上的高密度颗粒流化、混合颗粒流化和颗粒涂层过程。工艺模拟用于在宏观尺度上研究整个 FB-CVD 生产线。最后,揭示了多尺度耦合研究 FB-CVD 过程在核燃料颗粒工业制造中的巨大应用潜力。本文有助于流化床学术研究领域的发展。同时,对拓展 FB-CVD 的其他工业应用也具有启发和借鉴意义。
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