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Issue Highlights
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-03-09 DOI: 10.1002/cjce.25325
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引用次数: 0
Issue Highlights
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-02-03 DOI: 10.1002/cjce.25323
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引用次数: 0
Process simulation on oxy-fuel combustion of coal and biomass in a circulating fluidized bed
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-01-22 DOI: 10.1002/cjce.25600
Xuejiao Liu, Zecheng Liu, Yun Hu, Wenqi Zhong

Appropriately evaluating the gas–solid hydrodynamics and reaction kinetics of reactors within process simulation approach can provide more accurate and comprehensive techno-economic and environmental assessments, as well as more effective design and optimization for new processes and technologies. In this study, a one-dimensional process simulation of biomass and coal oxy-co-firing in a 100 kWth circulating fluidized bed was developed, with the models for gas–solid hydrodynamics and synergistic reactions of two fuels being established in Aspen Plus software. The effects of fuel properties, gas atmosphere, and operating parameters on the combustion process, flue gas products, and heat distributions in the bed were studied. Results show that the proposed process models can successfully describe the oxy-co-firing of coal and biomass in the furnace including the pyrolysis and the combustions of gaseous volatile and char. Increasing the oxygen concentration and biomass blending ratio will improve the combustions in dense phase region and obviously increase the heat release in this region. More heating surfaces should be arranged in the dense phase region when retrofitting an existing circulating fluidized bed (CFB) boiler with air combustion to be the oxy-fuel one. Additionally, the increase of oxygen concentration could reduce the emissions of pollutants such as CO and NOX, while the addition of biomass may bring a slight increase in NOX emission.

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引用次数: 0
Special section in honour of Professor Norman Epstein of the University of British Columbia
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-01-09 DOI: 10.1002/cjce.25599
João B. P. Soares
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引用次数: 0
Issue Highlights
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-01-07 DOI: 10.1002/cjce.25321
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引用次数: 0
Reliable modelling of the sulphur properties to calculate the process parameters of the Claus sulphur recovery plant
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2024-12-17 DOI: 10.1002/cjce.25573
Mohammad M. Ghiasi, Sohrab Zendehboudi, Amir H. Mohammadi, Mahdi Nikkhahi, Ali Lohi, Ioannis Chatzis

In order to handle the overwhelming effects of the removed hydrogen sulphide (H2S) from natural gas and industrial waste gases on the environment, H2S can be converted to elemental sulphur. Among the available processes for sulphur recovery, the most widely employed process is a modified Claus process. In this work, first, least square version of support vector machine (LS-SVM) approach is utilized for determining the properties of sulphur including heat of vaporization, heat of condensation (S6, S8), heat of dissociation (S6, S8), and heat capacity of equilibrium sulphur vapours as a function of temperature. An illustrative example is given to show the usefulness of the presented computer-based models with two parameters for designing and operation of the Claus sulphur recovery unit (SRU). According to the error analysis results, predicted values by the proposed intelligent models are in excellent agreement with the reported data in the literature for the aforementioned sulphur properties where the coefficient of determination (R2) is higher than 0.99 for all developed models. The average absolute relative deviation percent (%AARD) is less than 1.3 while predicting the heat capacity of equilibrium sulphur vapours. Other proposed models' predictions show less than 0.2% AARD from the target values. In addition, a mathematical algorithm on the basis of the Leverage approach is proposed to define the domain of applicability of the developed LS-SVM models. It was found that the presented models are statistically valid and the employed data points for developing the models are within the range of their applicability.

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引用次数: 0
Preface to the special issue section: Artificial intelligence and machine learning applications in chemical engineering
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2024-12-09 DOI: 10.1002/cjce.25572
Simant Upreti
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引用次数: 0
Issue Highlights 问题突出
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2024-12-04 DOI: 10.1002/cjce.25319
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引用次数: 0
Towards a more sustainable future: Transitioning from thermochemical to electrochemical processes in clean energy technologies relevant to hydrogen-containing fuels
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2024-11-28 DOI: 10.1002/cjce.25549
Jasna Jankovic, David P. Wilkinson

This review paper explores the transition from thermochemical to electrochemical processes in clean energy technologies, particularly focusing on hydrogen-containing fuels, namely hydrogen, ammonia, and methanol. The main characteristics of the thermochemical and electrochemical technologies are compared, followed by a focus on specific approaches in production of each of these e-fuels. Steam methane reforming, partial oxidation of hydrocarbons, coal and biomass gasification, as well as thermal decomposition and autothermal reforming processes are discussed for hydrogen thermochemical production. Electrochemical technologies for green hydrogen production are then described, including water electrolysis based on alkaline, proton exchange membrane, anion exchange, and solid oxide cells. The paper further compares the Haber–Bosch process with the electrochemical synthesis of ammonia, and discusses thermochemical technologies for methanol synthesis from syngas, comparing them to the two electrochemical approaches-electrochemical CO2 reduction and methane oxidation reaction. Additionally, approaches for extracting hydrogen from ammonia and methanol by electrochemical reforming are briefly discussed. The paper closes with the future prospects and challenges of the transition from the traditional thermochemical technologies to the more sustainable electrochemical processes. Despite the promising prospects of the electrochemical technologies, challenges such as high initial capital costs, the need for advanced materials, and scalability must be addressed. Ongoing research, policy incentives, and collaborative efforts are essential to overcome these barriers and facilitate the transition to a low-carbon economy. In the meantime, the integration of these technologies represents a transformative approach to chemical manufacturing and energy management, offering a pathway towards more sustainable and versatile industrial practices.

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引用次数: 0
Top 15 articles published in the CJCE in 2024
IF 1.6 4区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2024-11-20 DOI: 10.1002/cjce.25565
João B. P. Soares
<p>It gives me great pleasure to write the editorial of this virtual issue of the <i>CJCE</i>, which collects 15 articles published in 2024 with the highest number of full-text views. This is a great opportunity to thank our authors for their outstanding contributions to the CJCE and also to ‘take the pulse’ of our readers and find out what topics they considered more relevant in 2024.</p><p>These 15 articles cover many areas of chemical engineering—composites, carbon capture, circular-plastic economy, polymeric materials, experimental methods in chemical engineering, microfluidic devices, risk and safety, oil and gas, and educational aspects related to the future chemical engineering—and showcase the fascinating breadth of our profession.</p><p>The first article in this virtual special issue is part of the <i>Conversations in Chemical Engineering</i> special series. This series is dear to me because it attempts to change the way we write scientific papers in order to make them more accessible to a broader readership, not only to the conventional cadre of specialists. As I wrote not too long ago in an article entitled “Is It Time to Change How We Write Scientific Articles?,” ‘The only correct way to write an article is to express your ideas so clearly that after reading it, your readers would say, “Why didn't I think of this before?”’<sup>[</sup><span><sup>1</sup></span><sup>]</sup></p><p>In his contribution to the <i>Conversations in Chemical Engineering</i> special series, now included in this virtual issue, De France (Queen's University) captures the attention of his readers in the first sentence of his article on cellulose nanocrystal composites by asking them, ‘Just like jumbo shrimp, “liquid crystal” is an oxymoron—how can something be both a delicate, shapeless liquid and a robust, solid crystal?’<sup>[</sup><span><sup>2</sup></span><sup>]</sup> In his comprehensive and accessible review, the author introduces the basics of liquid crystals and self-assembly, and explains the main approaches used to form cellulose nanocrystals (CNC) based composite films, such as co-assembly, templating, and post-processing. He finishes his paper with his uniquely Canadian perspective on the current status, future prospects, and major challenges associated with the development of CNC-based chiral nematic composite materials.</p><p>Carbon capture—echoing our modern anxieties about climate change—has also been in the minds of our readers. In the second article in this virtual issue, Usas and Ricardez-Sandoval (University of Waterloo) review the state of CO<sub>2</sub> capture in Canada,<sup>[</sup><span><sup>3</sup></span><sup>]</sup> addressing the measures our nation is taking to address sustainable decarbonization in the context of carbon capture. The authors also suggest a new optimal framework for carbon capture implementation that accounts for environmental and social considerations.</p><p>When we think about sustainability these days, one of the first
我非常高兴能为这期虚拟期刊撰写社论,这期期刊收集了2024年发表的全文浏览量最高的15篇文章。这 15 篇文章涵盖了化学工程的多个领域--复合材料、碳捕集、循环-塑料经济、高分子材料、化学工程中的实验方法、微流体设备、风险与安全、石油与天然气,以及与未来化学工程相关的教育问题--展示了我们专业的迷人广度。这一系列文章对我来说非常重要,因为它试图改变我们撰写科学论文的方式,以便让更多的读者,而不仅仅是传统意义上的专家更容易接受它们。正如我不久前在一篇题为《是时候改变我们撰写科学论文的方式了吗?"'撰写文章的唯一正确方法就是清楚地表达自己的观点,让读者读完后会说:"为什么我以前没有想到这一点?'"[1]De France(皇后大学)为《化学工程对话》特辑撰写了一篇关于纤维素纳米晶体复合材料的文章,现在收录在本期虚拟刊物中,他在文章的第一句话就吸引了读者的注意力,他问读者:"就像巨型虾一样,'液晶'是一个矛盾体--怎么可能既是细腻、无形的液体,又是坚固的固体晶体呢?'[2]在这篇全面而通俗易懂的评论中,作者介绍了液晶和自组装的基础知识,并解释了用于形成基于纤维素纳米晶体 (CNC) 的复合薄膜的主要方法,例如共组装、模板化和后处理。最后,他以加拿大独特的视角阐述了基于 CNC 的手性向列复合材料的发展现状、未来前景和主要挑战。在本期虚拟刊物的第二篇文章中,Usas 和 Ricardez-Sandoval (滑铁卢大学)回顾了加拿大的二氧化碳捕集现状,[3] 阐述了我国在碳捕集背景下为解决可持续脱碳问题而采取的措施。作者还为碳捕集的实施提出了一个新的最佳框架,其中考虑到了环境和社会因素。如今,当我们考虑可持续发展时,首先想到的就是塑料对环境的影响。舒尔茨-内策尔(Schulze-Netzer)(挪威科技大学)针对令人担忧的 "塑料泛滥 "问题提出了一个可行的解决方案,即利用气化技术进行材料回收。大多数废弃塑料(约 73%)最终被填埋或管理不当,导致垃圾泛滥"。这些数字令人震惊,而大多数人可能并不了解塑料回收技术的局限性。Schulze-Netzer 解释了这些令人沮丧的数字背后的原因,指出了大多数机械回收方法的局限性,并特别指出蒸汽气化是回收混合塑料、受污染塑料和不可分类塑料的最有前途的方法之一。作者认为,蒸汽气化的优势可以显著提高回收率,并为生物一体化循环碳经济做出贡献。"化学工程中的实验方法 "系列文章由蒙特利尔理工大学的格雷戈里-帕蒂斯(Gregory Patience)组织撰写,是《化学工程》杂志过去几年来最成功的特别系列文章。我很高兴地发现,这个非凡的特别系列中的三篇文章也进入了 2024 年 CJCE 文章排行榜的前 15 名,这加强了我们的读者对这些文章的兴趣。在《化学工程中的实验方法》系列的第一篇文章中,Rivera-Quintero 等人回顾了卡尔-费休滴定法,这是一种广泛用于测量有机和无机化合物中水含量的方法,并解释了该方法的工作原理及其主要局限性[5]。文献计量分析将这些文章分为五组:光谱学、稳定性、温度、溶解度和混合物。
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