Momentum-resolved EELS and CL study on 1D-plasmonic crystal prepared by FIB method.

Akira Yasuhara, Masateru Shibata, Wakaba Yamamoto, Izzah Machfuudzoh, Sotatsu Yanagimoto, Takumi Sannomiya
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Abstract

We investigate a one-dimensional plasmonic crystal using momentum-resolved electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) techniques, which are complementary in terms of available optical information. The plasmonic crystal sample is fabricated from large aluminum grains through the focused ion beam method. This approach allows curving nanostructures with high crystallinity, providing platforms for detailed analysis of plasmonic nanostructures using both EELS and CL. The momentum-resolved EELS visualizes dispersion curves outside the light cone, confirming the existence of the surface plasmon polaritons and local modes, while the momentum-resolved CL mapping analysis identified these surface plasmon polaritons and local modes. Such synergetic approach of two electron-beam techniques offers full insights into both radiative and non-radiative optical properties in plasmonic or photonic structures.

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用 FIB 方法制备的一维等离子晶体的动量分辨 EELS 和 CL 研究。
我们利用动量分辨电子能量损失光谱(EELS)和阴极发光(CL)技术研究了一种一维等离子晶体(1D PlC),这两种技术在可用光学信息方面具有互补性。PlC 样品是通过聚焦离子束 (FIB) 方法从大型铝晶粒中制造出来的。这种方法可实现具有高结晶度的弯曲纳米结构,为使用 EELS 和 CL 对等离子纳米结构进行详细分析提供了平台。动量分辨 EELS 可观察到光锥外的色散曲线,证实了表面等离子体极化子 (SPP) 和局部模式的存在,而动量分辨 CL 绘图分析则确定了这些 SPP 和局部模式。通过两种电子束技术的协同作用,可以全面了解等离子体或光子结构中的辐射和非辐射光学特性。
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