ZnAl-LDH film for self-powered ultraviolet photodetection

IF 17.9 2区 材料科学 Q1 Engineering Nano Materials Science Pub Date : 2025-06-01 DOI:10.1016/j.nanoms.2024.05.001
Simin Sun , Yuan Zhang , Qiyue Gao , Nana Zhang , PingAn Hu , Wei Feng
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Abstract

Self-powered photoelectrochemical-type (PEC) ultraviolet photodetectors (UV PDs) have been rapidly developed owing to their low-cost fabrication and good photodetection. However, achieving high-performance and self-powered PEC UV PDs based on an individual material is still challenging. Therefore, developing more wide bandgap semiconductors for high-performance PEC UV PDs is attractive. Here, we demonstrate that ZnAl-LDH is suitable for self-powered PEC UV PDs with high responsivity and excellent wavelength selectivity for the first time. The responsivity is 29.25 ​mA/W (254 ​nm irradiation) and the UV/visible rejection ratio is 1037, surpassing most PEC UV PDs. Furthermore, the PEC UV PDs have fast response, good stability, and underwater optical communication capability. This work offers more chances for the development of high-performance PEC UV PDs and demonstrates the potential application of ZnAl-LDH in underwater optoelectronic devices.

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用于自供电紫外光检测的 ZnAl-LDH 薄膜
自供电型光电化学型紫外探测器(UV pd)因其制造成本低、光探测性能好而得到了迅速发展。然而,基于单个材料实现高性能和自供电的PEC UV pd仍然具有挑战性。因此,开发更多的宽禁带半导体用于高性能PEC UV pd是有吸引力的。本文首次证明了ZnAl-LDH适用于具有高响应性和优异波长选择性的自供电PEC UV pd。响应度为29.25 mA/W (254 nm辐照),UV/可见光抑制比为1037,超过了大多数PEC UV pd。此外,PEC UV pd具有响应快、稳定性好、水下光通信能力强等特点。这项工作为高性能PEC UV pd的发展提供了更多的机会,并展示了ZnAl-LDH在水下光电器件中的潜在应用。
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来源期刊
Nano Materials Science
Nano Materials Science Engineering-Mechanics of Materials
CiteScore
20.90
自引率
3.00%
发文量
294
审稿时长
9 weeks
期刊介绍: Nano Materials Science (NMS) is an international and interdisciplinary, open access, scholarly journal. NMS publishes peer-reviewed original articles and reviews on nanoscale material science and nanometer devices, with topics encompassing preparation and processing; high-throughput characterization; material performance evaluation and application of material characteristics such as the microstructure and properties of one-dimensional, two-dimensional, and three-dimensional nanostructured and nanofunctional materials; design, preparation, and processing techniques; and performance evaluation technology and nanometer device applications.
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