Forced ignition of cool, warm and hot flames in a laminar non-premixed counterflow of DME versus air

IF 5.3 2区 工程技术 Q2 ENERGY & FUELS Proceedings of the Combustion Institute Pub Date : 2024-01-01 DOI:10.1016/j.proci.2024.105222
Yan Wang , Yiqing Wang , Xinyi Chen , Shumeng Xie , Hannes Böttler , Arne Scholtissek , Christian Hasse , Zheng Chen
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Abstract

Recently, there has been great interest in the ignition of cool and warm flames (controlled by low-temperature chemistry, LTC, and intermediate-temperature chemistry, ITC, respectively) as they may have significant influence on the ignition and subsequent propagation of hot flame. However, it is still unclear how the flow affects the ignition of the cool/warm flame and their transition to the hot flame in a non-premixed fuel/oxidizer system. In this study, we conduct 2D simulations on the forced ignition of cool, warm and hot flames in a laminar, axisymmetric, non-premixed counterflow of dimethyl ether (DME) versus air. The objective is to assess the effects of flow on the ignition of cool, warm, and/or hot flames and the transition among them. Different ignition energies and strain rates are considered. It is found that the transient ignition process is mainly controlled by the extinction/transition limits and the minimum ignition energies of cool, warm and hot flames. When the strain rate is lower than the transition limits of cool and warm flames, all three flame types can be directly initiated but they eventually evolve into a hot flame. At intermediate strain rate between the transient limit and the extinction limit, quasi-steady cool and warm flames can be obtained without further transition to a hot flame. When the strain rate exceeds the extinction limit of cool and warm flames, only the hot flame can be ignited. An ignition regime diagram in terms of ignition energy and strain rate is proposed, in which different regimes for cool, warm and hot flames as well as transition among them are identified. Furthermore, the ignition of cool and warm flames in a non-premixed counterflow is shown to be very sensitive to ignition position as well as strain rate and ignition energy.

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在二甲醚与空气的层流非预混合逆流中强制点燃冷焰、暖焰和热焰
最近,人们对冷焰和暖焰(分别由低温化学反应(LTC)和中温化学反应(ITC)控制)的点燃产生了浓厚的兴趣,因为它们可能对热焰的点燃和随后的传播产生重大影响。然而,在非预混合燃料/氧化剂系统中,流动如何影响冷焰/暖焰的点燃及其向热焰的过渡仍不清楚。在本研究中,我们对二甲醚(DME)与空气的层流、轴对称、非预混逆流中冷焰、暖焰和热焰的强制点火进行了二维模拟。目的是评估流动对冷焰、暖焰和/或热焰点火的影响以及它们之间的过渡。考虑了不同的点火能量和应变率。研究发现,瞬态点火过程主要受控于冷焰、暖焰和热焰的熄灭/过渡极限和最小点火能量。当应变率低于冷焰和暖焰的过渡极限时,三种火焰都可以直接点燃,但最终都会演变成热焰。当应变速率介于瞬态极限和熄灭极限之间时,可获得准稳定的冷焰和暖焰,而不会进一步过渡到热焰。当应变速率超过冷焰和暖焰的熄灭极限时,只能点燃热焰。根据点火能量和应变率提出了点火机制图,其中确定了冷焰、暖焰和热焰的不同机制以及它们之间的过渡。此外,在非预混合逆流中,冷焰和暖焰的点火对点火位置、应变率和点火能量非常敏感。
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来源期刊
Proceedings of the Combustion Institute
Proceedings of the Combustion Institute 工程技术-工程:化工
CiteScore
7.00
自引率
0.00%
发文量
420
审稿时长
3.0 months
期刊介绍: The Proceedings of the Combustion Institute contains forefront contributions in fundamentals and applications of combustion science. For more than 50 years, the Combustion Institute has served as the peak international society for dissemination of scientific and technical research in the combustion field. In addition to author submissions, the Proceedings of the Combustion Institute includes the Institute''s prestigious invited strategic and topical reviews that represent indispensable resources for emergent research in the field. All papers are subjected to rigorous peer review. Research papers and invited topical reviews; Reaction Kinetics; Soot, PAH, and other large molecules; Diagnostics; Laminar Flames; Turbulent Flames; Heterogeneous Combustion; Spray and Droplet Combustion; Detonations, Explosions & Supersonic Combustion; Fire Research; Stationary Combustion Systems; IC Engine and Gas Turbine Combustion; New Technology Concepts The electronic version of Proceedings of the Combustion Institute contains supplemental material such as reaction mechanisms, illustrating movies, and other data.
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