Recent Progress and Future Prospects of Metal-Organic Frameworks for Adsorption, Separation and Catalytic Removal of NOx and N2O

IF 3.8 3区 化学 Q2 CHEMISTRY, PHYSICAL ChemCatChem Pub Date : 2024-06-13 DOI:10.1002/cctc.202400922
Ming-Wu Liu, Hao Zhang, Jing Li, Xiao-Chen Qi, Yu-Fen Wang, Jiandong Pang
{"title":"Recent Progress and Future Prospects of Metal-Organic Frameworks for Adsorption, Separation and Catalytic Removal of NOx and N2O","authors":"Ming-Wu Liu,&nbsp;Hao Zhang,&nbsp;Jing Li,&nbsp;Xiao-Chen Qi,&nbsp;Yu-Fen Wang,&nbsp;Jiandong Pang","doi":"10.1002/cctc.202400922","DOIUrl":null,"url":null,"abstract":"<p>Nitrogen oxides (NOx) are produced during the high-temperature combustion process of fossil fuels, which are considered as an atmospheric pollutant that can lead to significant environmental issues such as acid rain and photochemical smog. Therefore, it is essential to minimize the concentration of NO<sub>x</sub> in the atmosphere in order to protect the ecological environment upon which human beings depends. The integrated utilization of NO<sub>x</sub> removal technology results in environmentally harmless compounds, such as N<sub>2</sub> and H<sub>2</sub>O, through the processes like adsorption, separation, catalytic reduction and other methods. Metal-organic frameworks (MOFs) are seen as ideal candidates for addressing NO<sub>x</sub> pollution issues in the atmosphere due to their high specific surface area, ultrahigh porosity and unlimited modifiability. Herein, the latest research progress in MOFs and MOFs-derived materials related to NO<sub>x</sub> adsorption, separation and catalytic reduction is presented and summarized. Besides, some opportunities and problems need to be solved in this field are proposed and discussed.</p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":null,"pages":null},"PeriodicalIF":3.8000,"publicationDate":"2024-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ChemCatChem","FirstCategoryId":"92","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/cctc.202400922","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

Abstract

Nitrogen oxides (NOx) are produced during the high-temperature combustion process of fossil fuels, which are considered as an atmospheric pollutant that can lead to significant environmental issues such as acid rain and photochemical smog. Therefore, it is essential to minimize the concentration of NOx in the atmosphere in order to protect the ecological environment upon which human beings depends. The integrated utilization of NOx removal technology results in environmentally harmless compounds, such as N2 and H2O, through the processes like adsorption, separation, catalytic reduction and other methods. Metal-organic frameworks (MOFs) are seen as ideal candidates for addressing NOx pollution issues in the atmosphere due to their high specific surface area, ultrahigh porosity and unlimited modifiability. Herein, the latest research progress in MOFs and MOFs-derived materials related to NOx adsorption, separation and catalytic reduction is presented and summarized. Besides, some opportunities and problems need to be solved in this field are proposed and discussed.

Abstract Image

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
用于吸附、分离和催化去除氮氧化物和氧化亚氮的金属有机框架的最新进展和未来展望
氮氧化物(NOx)是化石燃料在高温燃烧过程中产生的,被认为是一种大气污染物,可导致酸雨和光化学烟雾等重大环境问题。因此,为了保护人类赖以生存的生态环境,必须最大限度地降低大气中氮氧化物的浓度。综合利用氮氧化物去除技术,通过吸附、分离、催化还原等过程,产生对环境无害的化合物,如 N2 和 H2O。金属有机框架(MOFs)因其高比表面积、超高孔隙率和无限可改性,被视为解决大气中氮氧化物污染问题的理想候选材料。本文介绍并总结了与氮氧化物吸附、分离和催化还原相关的 MOFs 及其衍生材料的最新研究进展。此外,还提出并讨论了该领域的一些机遇和亟待解决的问题。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
ChemCatChem
ChemCatChem 化学-物理化学
CiteScore
8.10
自引率
4.40%
发文量
511
审稿时长
1.3 months
期刊介绍: With an impact factor of 4.495 (2018), ChemCatChem is one of the premier journals in the field of catalysis. The journal provides primary research papers and critical secondary information on heterogeneous, homogeneous and bio- and nanocatalysis. The journal is well placed to strengthen cross-communication within between these communities. Its authors and readers come from academia, the chemical industry, and government laboratories across the world. It is published on behalf of Chemistry Europe, an association of 16 European chemical societies, and is supported by the German Catalysis Society.
期刊最新文献
Front Cover: Ethylene Dimerization, Isomerization and Trimerization: Mechanistic Insights into Competing Pathways on Metal–Organic Framework Supported Metal Hydrides (ChemCatChem 20/2024) Cover Feature: Economically competitive Organic Acid-Base mixtures as Catalysts for the Self-Condensation of Diols into Polyethers (ChemCatChem 20/2024) Retraction: Nanoporous Au/Ag Catalyzed Benzylic sp3C−H Oxidation of 9H-Fluorene Derivatives and Similar Molecules With TBHP Front Cover: Catalytic Relevance of Mg-Al-O Basic Centers in the Upgrade of Ethanol to n-Butanol (ChemCatChem 19/2024) Cover Feature: Supported Cobalt Oxide Nanoparticles: The Influence of Mesoporous Materials and their Role in Methyl Phenyl Sulfide Oxidation Reactions (ChemCatChem 19/2024)
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1