Asymmetric electrostatic dodecapole: compact bandpass filter with low aberrations for momentum microscopy.

IF 2.5 3区 物理与天体物理 Journal of Synchrotron Radiation Pub Date : 2024-07-01 Epub Date: 2024-06-20 DOI:10.1107/S1600577524003540
O Tkach, S Chernov, S Babenkov, Y Lytvynenko, O Fedchenko, K Medjanik, D Vasilyev, A Gloskowskii, C Schlueter, H J Elmers, G Schönhense
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Abstract

Imaging energy filters in photoelectron microscopes and momentum microscopes use spherical fields with deflection angles of 90°, 180° and even 2 × 180°. These instruments are optimized for high energy resolution, and exhibit image aberrations when operated in high transmission mode at medium energy resolution. Here, a new approach is presented for bandpass-filtered imaging in real or reciprocal space using an electrostatic dodecapole with an asymmetric electrode array. In addition to energy-dispersive beam deflection, this multipole allows aberration correction up to the third order. Here, its use is described as a bandpass prefilter in a time-of-flight momentum microscope at the hard X-ray beamline P22 of PETRA III. The entire instrument is housed in a straight vacuum tube because the deflection angle is only 4° and the beam displacement in the filter is only ∼8 mm. The multipole is framed by transfer lenses in the entrance and exit branches. Two sets of 16 different-sized entrance and exit apertures on piezomotor-driven mounts allow selection of the desired bandpass. For pass energies between 100 and 1400 eV and slit widths between 0.5 and 4 mm, the transmitted kinetic energy intervals are between 10 eV and a few hundred electronvolts (full width at half-maximum). The filter eliminates all higher or lower energy signals outside the selected bandpass, significantly improving the signal-to-background ratio in the time-of-flight analyzer.

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不对称静电十二极:用于动量显微镜的低像差紧凑型带通滤波器。
光电子显微镜和动量显微镜中的成像能量滤波器使用偏转角为 90°、180° 甚至 2 × 180°的球形场。这些仪器针对高能量分辨率进行了优化,在中等能量分辨率下以高传输模式运行时会出现图像畸变。这里介绍的是一种新方法,利用带有非对称电极阵列的静电十二极在实空间或倒易空间进行带通滤波成像。除了能量色散光束偏转外,这种多极还能进行高达三阶的像差校正。这里介绍的是它在 PETRA III 硬 X 射线光束线 P22 的飞行时间动量显微镜中作为带通预滤波器的用途。由于偏转角仅为 4°,滤波器中的光束位移仅为 ∼ 8 毫米,因此整个仪器安装在一个直的真空管中。多极子由入口和出口分支的传递透镜构成。在压电电机驱动的支架上有两组 16 个不同大小的入口和出口孔径,可以选择所需的带通。当通过能量在 100 到 1400 eV 之间,狭缝宽度在 0.5 到 4 mm 之间时,传输的动能区间在 10 eV 到几百电子伏特(半最大全宽)之间。滤波器可以消除所选带通外的所有较高或较低能量信号,从而显著提高飞行时间分析仪的信噪比。
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来源期刊
Journal of Synchrotron Radiation
Journal of Synchrotron Radiation INSTRUMENTS & INSTRUMENTATIONOPTICS&-OPTICS
CiteScore
5.60
自引率
12.00%
发文量
289
审稿时长
1 months
期刊介绍: Synchrotron radiation research is rapidly expanding with many new sources of radiation being created globally. Synchrotron radiation plays a leading role in pure science and in emerging technologies. The Journal of Synchrotron Radiation provides comprehensive coverage of the entire field of synchrotron radiation and free-electron laser research including instrumentation, theory, computing and scientific applications in areas such as biology, nanoscience and materials science. Rapid publication ensures an up-to-date information resource for scientists and engineers in the field.
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