Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign

IF 5.2 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES Atmospheric Chemistry and Physics Pub Date : 2024-06-24 DOI:10.5194/acp-24-7179-2024
Britta Schäfer, Robert Oscar David, Paraskevi Georgakaki, Julie Thérèse Pasquier, Georgia Sotiropoulou, Trude Storelvmo
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Abstract

Abstract. The representation of Arctic clouds and their phase distributions, i.e., the amount of ice and supercooled water, influences predictions of future Arctic warming. Therefore, it is essential that cloud phase is correctly captured by models in order to accurately predict the future Arctic climate. Ice crystal formation in clouds happens through ice nucleation (primary ice production) and ice multiplication (secondary ice production). In common weather and climate models, rime splintering is the only secondary ice production process included. In addition, prescribed number concentrations of cloud condensation nuclei or cloud droplets and ice-nucleating particles are often overestimated in Arctic environments by standard model configurations. This can lead to a misrepresentation of the phase distribution and precipitation formation in Arctic mixed-phase clouds, with important implications for the Arctic surface energy budget. During the Ny-Ålesund Aerosol Cloud Experiment (NASCENT), a holographic probe mounted on a tethered balloon took in situ measurements of number and mass concentrations of ice crystals and cloud droplets in Svalbard, Norway, during fall 2019 and spring 2020. In this study, we choose one case study from this campaign that shows evidence of strong secondary ice production and use the Weather Research and Forecasting (WRF) model to simulate it at a high vertical and spatial resolution. We test the performance of different microphysical parametrizations and apply a new state-of-the-art secondary ice parametrization. We find that agreement with observations highly depends on the prescribed cloud condensation nuclei/cloud droplet and ice-nucleating particle concentrations and requires an enhancement of secondary ice production processes. Lowering mass mixing ratio thresholds for rime splintering inside the Morrison microphysics scheme is crucial to enable secondary ice production and thereby match observations for the right reasons. In our case, rime splintering is required to initiate collisional breakup. The simulated contribution from collisional breakup is larger than that from droplet shattering. Simulating ice production correctly for the right reasons is a prerequisite for reliable simulations of Arctic mixed-phase cloud responses to future temperature or aerosol perturbations.
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尼-埃勒松德气溶胶云实验(NASCENT)活动中北极混合相云情况下的初级和次级冰生产模拟
摘要北极云及其云相分布(即冰和过冷却水的数量)的表示影响对未来北极变暖的预测。因此,模型必须正确捕捉云相,以准确预测未来北极气候。云中冰晶的形成是通过冰核化(一次产冰)和冰增殖(二次产冰)进行的。在常见的天气和气候模型中,冰渣分裂是唯一包含的二次产冰过程。此外,标准模式配置通常会高估北极环境中云凝结核或云滴和成冰粒子的规定数量浓度。这可能导致北极混合相云中的相分布和降水形成被错误地描述,从而对北极地表能量预算产生重要影响。在 Ny-Ålesund 气溶胶云实验(NASCENT)期间,一个安装在系留气球上的全息探测器于 2019 年秋季和 2020 年春季在挪威斯瓦尔巴群岛对冰晶和云滴的数量和质量浓度进行了实地测量。在本研究中,我们从这次活动中选择了一个案例研究,该案例显示了强烈的二次产冰现象,并使用天气研究与预报(WRF)模型以较高的垂直和空间分辨率对其进行了模拟。我们测试了不同微物理参数的性能,并应用了最新的二次结冰参数。我们发现,与观测结果的一致性在很大程度上取决于规定的云凝结核/云滴和成冰粒子浓度,并且需要增强二次冰生成过程。在莫里森微物理方案中,降低云泥分裂的质量混合比阈值对于实现二次产冰至关重要,从而以正确的理由与观测结果相吻合。在我们的研究中,石灰劈裂是引发碰撞破裂的必要条件。碰撞破裂的模拟贡献大于液滴破碎的模拟贡献。以正确的理由正确模拟冰的生成是可靠模拟北极混合相云对未来温度或气溶胶扰动响应的前提条件。
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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