Satellite quantification of methane emissions from South American countries: A high-resolution inversion of TROPOMI and GOSAT observations

IF 5.2 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES Atmospheric Chemistry and Physics Pub Date : 2024-06-24 DOI:10.5194/egusphere-2024-1763
Sarah E. Hancock, Daniel Jacob, Zichong Chen, Hannah Nesser, Aaron Davitt, Daniel J. Varon, Melissa P. Sulprizio, Nicholas Balasus, Lucas A. Estrada, James D. East, Elise Penn, Cynthia A. Randles, John Worden, Ilse Aben, Robert J. Parker, Joannes D. Maasakkers
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Abstract

Abstract. We use 2021 TROPOMI and GOSAT satellite observations of atmospheric methane in an analytical inversion to quantify national methane emissions from South America at up to 25 km × 25 km resolution. From the inversion, we derive optimal posterior estimates of methane emissions correcting the national anthropogenic emission inventories reported by individual countries to the United Nations Framework Convention on Climate Change (UNFCCC) and taken here as prior estimates. We also evaluate two alternative wetland emission inventories (WetCHARTs and LPJ-wsl) as prior estimates. Our best posterior estimates for wetland emissions are consistent with previous inventories for the Amazon but lower for the Pantanal and higher for the Parana. Our best posterior estimate of South American anthropogenic emissions is 48 (41–56) Tg a-1, where numbers in parentheses are the range from our inversion ensemble. This is 55 % higher than UNFCCC reports and is dominated by livestock (65 % of anthropogenic total). We find that TROPOMI and GOSAT observations can effectively optimize and separate national emissions by sector for 10 of the 13 countries and territories in the region, 7 of which account for 93 % of continental anthropogenic emissions: Brazil (19 (16–23) Tg a−1), Argentina (9.2 (7.9–11) Tg a−1 ), Venezuela (7.0 (5.5-9.9) Tg a−1), Colombia (5.0 (4.4–6.7) Tg a−1), Peru (2.4 (1.6–3.9) Tg a−1), Bolivia (0.96 (0.66–1.2) Tg a−1), and Paraguay (0.93 (0.88 – 1.0) Tg a−1). Our estimates align with UNFCCC reports for Brazil, Bolivia, and Paraguay, but are significantly higher for other countries. Emissions in all countries are dominated by livestock (mainly enteric fermentation) except for oil/gas in Venezuela and landfills in Peru. Methane intensities from the oil/gas industry are high in Venezuela (33 %), Colombia (6.5 %) and Argentina (5.9 %). Country-average emission factors for enteric fermentation from cattle in UNFCCC reports are in the range 46–60 kg head-1 a-1, close to the IPCC Tier 1 estimate which is mostly based on data from Brazil. Our inversion yields cattle enteric fermentation emission factors consistent with the UNFCCC reports for Brazil and Bolivia but a factor of two higher for other countries. The discrepancy for Argentina can be corrected by using IPCC Tier 2 emission estimates accounting for high milk production.
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南美洲国家甲烷排放的卫星量化:TROPOMI 和 GOSAT 观测数据的高分辨率反演
摘要。我们在分析反演中使用了 2021 年 TROPOMI 和 GOSAT 卫星对大气甲烷的观测数据,以 25 km × 25 km 的分辨率量化了南美洲各国的甲烷排放量。通过反演,我们得出了甲烷排放的最优后验估计值,修正了各个国家向《联合国气候变化框架公约》(UNFCCC)报告的国家人为排放清单,并将其作为先验估计值。我们还评估了作为先验估计值的两个备选湿地排放清单(WetCHARTs 和 LPJ-wsl)。我们对湿地排放的最佳后验估计值与之前的亚马逊湿地排放清单一致,但对潘塔纳尔湿地排放的估计值较低,对巴拉那湿地排放的估计值较高。我们对南美洲人为排放的最佳后验估计值为 48 (41-56) Tg a-1,括号中的数字为反演集合的范围。这比《联合国气候变化框架公约》的报告高出 55%,并且以畜牧业为主(占人为排放总量的 65%)。我们发现,在该地区的 13 个国家和地区中,TROPOMI 和 GOSAT 观测数据可有效优化和分离 10 个国家和地区的各部门排放量,其中 7 个国家和地区的排放量占大陆人为排放量的 93%:巴西 (19 (16-23) Tg a-1)、阿根廷 (9.2 (7.9-11) Tg a-1)、委内瑞拉 (7.0 (5.5-9.9) Tg a-1)、哥伦比亚 (5.0 (4.4-6. 7) Tg a-1)、印度 (9.2 (7.9-11) Tg a-1)。7) Tg a-1)、秘鲁(2.4 (1.6-3.9) Tg a-1)、玻利维亚(0.96 (0.66-1.2) Tg a-1)和巴拉圭(0.93 (0.88 - 1.0) Tg a-1)。我们对巴西、玻利维亚和巴拉圭的估算与《联合国气候变化框架公约》报告一致,但对其他国家的估算要高得多。除委内瑞拉的石油/天然气和秘鲁的垃圾填埋场外,所有国家的甲烷排放均以畜牧业(主要是肠道发酵)为主。石油/天然气行业的甲烷强度在委内瑞拉(33%)、哥伦比亚(6.5%)和阿根廷(5.9%)很高。联合国气候变化框架公约》(UNFCCC)报告中各国牛肠内发酵的平均排放因子在 46-60 千克头-1 a-1 之间,接近 IPCC 第 1 级估计值,而 IPCC 第 1 级估计值主要基于巴西的数据。我们的反演结果显示,巴西和玻利维亚的牛肠内发酵排放因子与《联合国气候变化框架公约》报告一致,但其他国家则高出 2 倍。阿根廷的差异可通过使用 IPCC 第 2 级排放估计值(考虑到高牛奶产量)来纠正。
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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