π-π Stacked Nigrosine@Carbon Nanotube Nanocomposite as an All-in-One Additive for High Energy Flexible Batteries.

IF 15.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY ACS Nano Pub Date : 2024-06-25 DOI:10.1021/acsnano.4c04624
Zhihao Xing, Shihui Zou, Cong Ma, Qiangqiang Qiao, Xiaohan Cai, Ke Yue, Juxin Yue, Chunyi Zhou, Jiale Zheng, Yao Wang, Jianmin Luo, Huadong Yuan, Jianwei Nai, Xinyong Tao, Yujing Liu
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Abstract

The pursuit of high energy density in lithium batteries has driven the development of efficient electrodes with low levels of inactive components. Herein, a facile approach involving the use of π-π stacked nigrosine@carbon nanotube nanocomposites as an all-in-one additive for a LiFePO4 cathode has been developed. This design significantly reduces the proportion of inactive substances within the cathode, resulting in a battery that exhibits a high specific capacity of 143 mAh g-1 at a 1 C rate and shows commendable cyclic performance. Furthermore, the elimination of rigid current collectors endows the electrode with flexibility, offering avenues for future wearable energy storage devices.

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作为高能柔性电池多功能添加剂的π-π堆叠奈格里索@碳纳米管纳米复合材料。
对锂电池高能量密度的追求推动了低非活性成分高效电极的发展。在此,我们开发了一种简便的方法,即使用π-π堆叠黑氨酸@碳纳米管纳米复合材料作为磷酸铁锂阴极的一体化添加剂。这种设计大大降低了阴极中非活性物质的比例,使电池在 1 C 速率下的比容量高达 143 mAh g-1,并显示出令人称道的循环性能。此外,由于消除了刚性电流收集器,电极具有了灵活性,为未来的可穿戴储能设备提供了途径。
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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