Absolute Method for Measuring Environmental Radioactive Materials Using Imaging Plates.

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-10-01 Epub Date: 2024-06-29 DOI:10.1097/HP.0000000000001818
Mori Yutaro, Isobe Tomonori, Takei Hideyuki, Yoshimura Yosuke, Ide Yasuwo, Sugaya Keito, Sajyrau Gudetyjum, Sakae Takeji
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Abstract

Abstract: We had previously developed a measurement method using an imaging plate (IP) to evaluate and address surface contamination caused by the release of radioactive materials during the Fukushima nuclear accident. The measurement units for the surface contamination density were in relative values [described as relative luminescence levels measured in luminescence arbitrary units (LAU)], but the evaluation was required in absolute values, such as Bq cm -2 , to enable appropriate control of exposure doses. This study establishes a method for converting the IP measurements of surface contamination density due to environmental radioactivity into absolute values. Soil contaminated with radioactive materials from the Fukushima nuclear accident was collected to create a working reference material (WRM). The conversion coefficient for surface contamination density was calculated using the WRM values measured with an IP and high-purity germanium detectors. The IP measurement values were converted into the surface contamination density using the conversion coefficient. The WRM values measured with the IP and high-purity germanium detectors were 324.1 LAU and 32.22 ± 2.27 Bq cm -2 , respectively. The surface contamination density conversion factor was calculated as 0.0994. The surface contamination density on the roof of the Tsukuba City facility was re-evaluated using the conversion factor. The average value of 29,972 Bq m -2 matched the amount of radioactive material fallen in Tsukuba City. By standardizing the measurement conditions for surface contamination when using IPs, we successfully quantified the surface contamination density with an accuracy comparable to that of conventional methods. This method is expected to make a significant contribution to efficient radiation safety management.

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使用成像板测量环境放射性物质的绝对方法。
摘要:我们之前开发了一种使用成像板(IP)的测量方法,用于评估和处理福岛核事故期间放射性物质释放造成的表面污染。表面污染密度的测量单位是相对值[描述为以发光任意单位(LAU)测量的相对发光水平],但评估需要绝对值,如 Bq cm-2,以便适当控制照射剂量。本研究建立了一种方法,可将环境放射性导致的地表污染密度的 IP 测量值转换为绝对值。收集了福岛核事故中受到放射性物质污染的土壤,以创建工作参考材料(WRM)。使用 IP 和高纯锗探测器测量的 WRM 值计算了表面污染密度的转换系数。使用转换系数将 IP 测量值转换为表面污染密度。使用 IP 和高纯锗探测器测得的表面污染密度值分别为 324.1 LAU 和 32.22 ± 2.27 Bq cm-2。经计算,表面污染密度换算系数为 0.0994。使用转换系数重新评估了筑波市设施屋顶的表面污染密度。29,972 Bq m-2 的平均值与筑波市放射性物质的降落量相符。通过在使用 IPs 时对表面污染的测量条件进行标准化,我们成功地量化了表面污染密度,其精确度与传统方法相当。这种方法有望为高效的辐射安全管理做出重大贡献。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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