Pasquale Sellitto, Redha Belhadji, Bernard Legras, Aurélien Podglajen, Clair Duchamp
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引用次数: 0
Abstract
Abstract. The Hunga volcano violently erupted on January 15th, 2022, and produced the largest stratospheric aerosol layer perturbation of the last 30 years. One notable effect of the Hunga eruption was the significant modification of the size distribution (SD) of the stratospheric aerosol layer with respect to background conditions and other recent moderate stratospheric eruptions, with larger mean particles size and smaller SD spread for Hunga. Starting from satellite-based SD retrievals, and the assumption of pure sulphate aerosol layers, in this work we calculate the optical properties of both background and Hunga-perturbed stratospheric aerosol scenarios using a Mie code. We found that the intensive optical properties of the stratospheric aerosol layer (i.e., single scattering albedo, asymmetry parameter, aerosol extinction per unit mass and the broad-band average Ångström exponent) were not significantly perturbed by the Hunga eruption, with respect to background conditions. The calculated Ångström exponent was found consistent with multi-instrument satellite observations of the same parameter. Thus, the basic impact of the Hunga eruption on the optical properties of the stratospheric aerosol layer was an increase of the stratospheric aerosol extinction (or optical depth), without any modification of the shortwave and longwave relative absorption, angular scattering and broad-band spectral trend of the extinction, with respect to background. This highlights a marked difference of the Hunga perturbation of the stratospheric aerosol layer and those from other larger stratospheric eruptions, like Pinatubo 1991 and El Chichon 1982. With simplified radiative forcing estimations, we show that the Hunga eruption produced an aerosol layer likely 3–10 times more effective in producing a net cooling of the climate system with respect to Pinatubo and El Chichon eruptions, due to more effective shortwave scattering. As intensive optical properties are seldom directly measured, e.g. from satellite, our calculations can support the estimation of radiative effects for the Hunga eruption with climate or offline radiative models.
期刊介绍:
Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere.
The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.