Application of Johnson's approximation in finite element modeling for electric field-dependent materials

IF 1.8 4区 材料科学 Q2 MATERIALS SCIENCE, CERAMICS International Journal of Applied Ceramic Technology Pub Date : 2024-06-20 DOI:10.1111/ijac.14824
Rassell C. D'Silva Green, Graham Dale, Garry McLaughlin, Maureen Strawhorne, Derek C. Sinclair, Julian S. Dean
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Abstract

Johnson's approximation is implemented in a finite element code to simulate the electric field dependence of a core–shell microstructure material. We show how the microstructure, based here on a 50:50 volume fraction, influences the measured effective permittivity as a function of applied voltage. Using a Johnson's parameter of β = 1.0 × 1010 Vm5/C3, verified from commercial BaTiO3-based multilayer ceramic capacitors (MLCC), we show how the microstructure and the difference in core and shell conductivities alter the local fields generated and how this influences the voltage dependence of the effective permittivity. Systems that comprise a conductive core-like material surrounded by a resistive shell experience little or modest voltage dependence due to the shell material providing shielding to large electric fields within the cores. Conversely, if the core material is more resistive than the shell material, substantial voltage dependence occurs with simulations showing over a 50% decrease in the effective permittivity. These simulations give improved understanding of voltage dependence and provide a method to help guide the design of future materials for MLCCs with improved performance.

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约翰逊近似在电场相关材料有限元建模中的应用
约翰逊近似在有限元代码中得以实现,以模拟核壳微结构材料的电场依赖性。我们展示了基于 50:50 体积分数的微结构如何影响测量到的有效介电常数与外加电压的函数关系。我们使用从基于 BaTiO3 的商用多层陶瓷电容器 (MLCC) 中验证的约翰逊参数 β = 1.0 × 1010 Vm5/C3,展示了微结构以及芯壳电导率的差异如何改变产生的局部场,以及这如何影响有效介电常数的电压依赖性。由于外壳材料能屏蔽磁芯内的大电场,因此由类似导电磁芯的材料和电阻外壳组成的系统几乎不会产生电压依赖性。相反,如果内核材料的电阻比外壳材料大,则会出现严重的电压依赖性,模拟结果显示有效介电常数会下降 50%以上。这些模拟使人们对电压依赖性有了更深入的了解,并提供了一种方法,有助于指导未来 MLCC 材料的设计,提高其性能。
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来源期刊
International Journal of Applied Ceramic Technology
International Journal of Applied Ceramic Technology 工程技术-材料科学:硅酸盐
CiteScore
3.90
自引率
9.50%
发文量
280
审稿时长
4.5 months
期刊介绍: The International Journal of Applied Ceramic Technology publishes cutting edge applied research and development work focused on commercialization of engineered ceramics, products and processes. The publication also explores the barriers to commercialization, design and testing, environmental health issues, international standardization activities, databases, and cost models. Designed to get high quality information to end-users quickly, the peer process is led by an editorial board of experts from industry, government, and universities. Each issue focuses on a high-interest, high-impact topic plus includes a range of papers detailing applications of ceramics. Papers on all aspects of applied ceramics are welcome including those in the following areas: Nanotechnology applications; Ceramic Armor; Ceramic and Technology for Energy Applications (e.g., Fuel Cells, Batteries, Solar, Thermoelectric, and HT Superconductors); Ceramic Matrix Composites; Functional Materials; Thermal and Environmental Barrier Coatings; Bioceramic Applications; Green Manufacturing; Ceramic Processing; Glass Technology; Fiber optics; Ceramics in Environmental Applications; Ceramics in Electronic, Photonic and Magnetic Applications;
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