Comparative Analysis of the Chemical Composition of Surface and Groundwater in the Poyang Lake Catchment Area (China)

IF 0.3 Q4 GEOGRAPHY Geography and Natural Resources Pub Date : 2024-07-04 DOI:10.1134/s187537282470015x
D. Zhou, H. Yang, O. G. Savichev, K. Jin, Y. Wu, A. A. Khvashchevskaya
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Abstract

This paper analyzes data on the chemical composition of wetland waters, groundwaters, and river waters in the catchment area of Poyang Lake, which were obtained in the course of Russian–Chinese hydrogeochemical studies in 2013–2022. The bulk of the laboratory work was carried out at Tomsk Polytechnic University using the mass spectrometric method with inductively coupled plasma. It is shown that wetlands that are not used economically are a source of organic substances and their transformation products entering the groundwater of the upper hydrodynamic zone. An anthropogenic impact on surface and groundwaters has also been established, which manifests itself in a rather sharp increase in the concentrations of certain chemical elements and their compounds. However, at the same time, a significant ability of the region’s water bodies to self-purify has been revealed. Thus, in the low-water periods of 2019 and 2022, a decrease in the contents of As, Cd, Ni, Sb, V, Mo, and W in the waters of the Jinjiang River was noted, which is 17–120 times and more just 100–200 m downstream from wastewater outlets. Based on the analysis of measurement results, thermodynamic calculations, mathematical modeling of hydrogeochemical processes, and published materials of other authors, it is concluded that the most likely explanation for this ability is a combination of the following factors: the precipitation of poorly soluble substances (calcium and magnesium humates and carbonates and clay minerals) with the total content of dissolved salts amounting to more than 300–400 mg/dm3; the coprecipitation of a number of microelements, which increases with a decrease in the effective diameter of sediment particles (0.003 mm or less); and the involvement of substances removed from the solution in biogeochemical processes, the intensity of which increases under favorable climatic conditions (such as in the catchment area of Poyang Lake).

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鄱阳湖集水区地表水和地下水化学成分对比分析(中国)
摘要 本文分析了 2013-2022 年中俄水文地球化学研究过程中获得的有关鄱阳湖集水区湿地水、地下水和河水化学成分的数据。大部分实验室工作是在托木斯克理工大学使用电感耦合等离子体质谱法进行的。研究表明,未被经济利用的湿地是有机物质及其转化产物进入上游水动力区地下水的来源。人类活动对地表水和地下水的影响也已得到证实,表现为某些化学元素及其化合物的浓度急剧上升。但与此同时,该地区水体的自净能力也得到了证实。因此,在 2019 年和 2022 年的枯水期,锦江水体中的砷、镉、镍、锑、钒、钼和钨的含量都有所下降,仅在污水排放口下游 100-200 米处,下降幅度就达到 17-120 倍以上。根据对测量结果、热力学计算、水文地质化学过程数学模型和其他作者发表的资料的分析,得出结论认为,这种能力最有可能是由以下因素共同造成的:溶解性差的物质(钙镁腐殖酸盐和碳酸盐以及粘土矿物)的沉淀,其溶解盐的总含量超过 300-400 mg/dm3;一些微量元素的共沉淀,这种共沉淀随着沉积物颗粒有效直径的减小而增加(0.003 毫米或更小);从溶液中去除的物质参与生物地球化学过程,在有利的气候条件下(如在鄱阳湖集水区),这种参与的强度会增加。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
CiteScore
0.50
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0.00%
发文量
24
期刊介绍: Geography and Natural Resources  publishes information on research results in the field of geographical studies of nature, the economy, and the population. It provides ample coverage of the geographical aspects related to solving major economic problems, with special emphasis on regional nature management and environmental protection, geographical forecasting, integral regional research developments, modelling of natural processes, and on the advancement of mapping techniques. The journal publishes contributions on monitoring studies, geographical research abroad, as well as discussions on the theory of science.
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