{"title":"Measuring colloidomer hydrodynamics with holographic video microscopy","authors":"Jatin Abacousnac, Jasna Brujic, David G. Grier","doi":"10.1103/physreve.110.014605","DOIUrl":null,"url":null,"abstract":"In-line holographic video microscopy records a wealth of information about the microscopic structure and dynamics of colloidal materials. Powerful analytical techniques are available to retrieve that information when the colloidal particles are well separated. Large assemblies of close-packed particles create holograms that are substantially more challenging to interpret. We demonstrate that Rayleigh-Sommerfeld back propagation is useful for analyzing holograms of colloidomer chains, close-packed linear assemblies of micrometer-scale emulsion droplets. Colloidomers are fully flexible chains and undergo three-dimensional configurational changes under the combined influence of random thermal forces and hydrodynamic forces. We demonstrate the ability of holographic reconstruction to track these changes as colloidomers sediment through water in a horizontal slit pore. Comparing holographically measured configurational trajectories with predictions of hydrodynamic models both validates the analytical technique for this valuable class of self-organizing materials and also provides insights into the influence of geometric confinement on colloidomer hydrodynamics.","PeriodicalId":20085,"journal":{"name":"Physical review. E","volume":null,"pages":null},"PeriodicalIF":2.4000,"publicationDate":"2024-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical review. E","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physreve.110.014605","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Mathematics","Score":null,"Total":0}
引用次数: 0
Abstract
In-line holographic video microscopy records a wealth of information about the microscopic structure and dynamics of colloidal materials. Powerful analytical techniques are available to retrieve that information when the colloidal particles are well separated. Large assemblies of close-packed particles create holograms that are substantially more challenging to interpret. We demonstrate that Rayleigh-Sommerfeld back propagation is useful for analyzing holograms of colloidomer chains, close-packed linear assemblies of micrometer-scale emulsion droplets. Colloidomers are fully flexible chains and undergo three-dimensional configurational changes under the combined influence of random thermal forces and hydrodynamic forces. We demonstrate the ability of holographic reconstruction to track these changes as colloidomers sediment through water in a horizontal slit pore. Comparing holographically measured configurational trajectories with predictions of hydrodynamic models both validates the analytical technique for this valuable class of self-organizing materials and also provides insights into the influence of geometric confinement on colloidomer hydrodynamics.
期刊介绍:
Physical Review E (PRE), broad and interdisciplinary in scope, focuses on collective phenomena of many-body systems, with statistical physics and nonlinear dynamics as the central themes of the journal. Physical Review E publishes recent developments in biological and soft matter physics including granular materials, colloids, complex fluids, liquid crystals, and polymers. The journal covers fluid dynamics and plasma physics and includes sections on computational and interdisciplinary physics, for example, complex networks.