Data-driven framework for general explicit formula of ionic thermoregulated osmotic energy conversion based on similarity principle and deep learning

IF 16.8 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Nano Energy Pub Date : 2024-07-02 DOI:10.1016/j.nanoen.2024.109955
Huangyi Zhu, Zhiguo Qu, Ziling Guo, Jianfei Zhang
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Abstract

Ionic thermoregulated osmotic energy conversion in nanochannels synergistically utilizes osmotic and thermal energy for power generation based on ionic selective transport in charged nano-membranes under salinity gradients and thermal regulations. Currently, no explicit general dimensionless formulas exist that reflect the relationship between impact factors and performance to guide performance designs. In this study, data-driven insight is presented to establish a framework for obtaining explicit and general relational expressions based on data augmentation using the similarity principle and deep learning. The original database is derived from a finite element simulation with 10,000 dimensional samples, then augmented to 30,000 dimensional samples via similarity principle-based data augmentation. Subsequently, a deep neural network model with decay algorithms is employed to expand the database to new 300,000 dimensional samples with a prediction accuracy exceeding 98 %, which are further converted to dimensionless forms for multiple linear regression. Three dimensionless and explicit formulas for the electrical potential, output power, and energy conversion efficiency are obtained, which indicate determination coefficients of 0.91, 0.93, and 0.92, respectively. Furthermore, considering actual experimental and application situations, the modified dimensionless formula of the output power predicts the experimental results with an average error of 7.80 %. This study efficiently alleviates experimental burden and facilitates engineering applications.

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基于相似性原理和深度学习的离子热调节渗透能量转换通用显式公式的数据驱动框架
在盐度梯度和热调节条件下,纳米通道中的离子热调节渗透能量转换基于带电纳米膜中的离子选择性传输,协同利用渗透和热能进行发电。目前,还没有明确的通用无量纲公式来反映影响因素与性能之间的关系,以指导性能设计。本研究提出了数据驱动的见解,以建立一个框架,利用相似性原理和深度学习,在数据增强的基础上获得明确的通用关系表达式。原始数据库来自有限元模拟,包含 10,000 个维度样本,然后通过基于相似性原理的数据扩增,扩增到 30,000 个维度样本。随后,采用带有衰减算法的深度神经网络模型,将数据库扩展到新的 300,000 个维度样本,预测准确率超过 98%,并进一步转换为无维度形式,用于多元线性回归。得到了电动势、输出功率和能量转换效率的三个无量纲和显式公式,其确定系数分别为 0.91、0.93 和 0.92。此外,考虑到实际实验和应用情况,修正后的输出功率无量纲公式预测实验结果的平均误差为 7.80%。这项研究有效地减轻了实验负担,促进了工程应用。
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来源期刊
Nano Energy
Nano Energy CHEMISTRY, PHYSICAL-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
30.30
自引率
7.40%
发文量
1207
审稿时长
23 days
期刊介绍: Nano Energy is a multidisciplinary, rapid-publication forum of original peer-reviewed contributions on the science and engineering of nanomaterials and nanodevices used in all forms of energy harvesting, conversion, storage, utilization and policy. Through its mixture of articles, reviews, communications, research news, and information on key developments, Nano Energy provides a comprehensive coverage of this exciting and dynamic field which joins nanoscience and nanotechnology with energy science. The journal is relevant to all those who are interested in nanomaterials solutions to the energy problem. Nano Energy publishes original experimental and theoretical research on all aspects of energy-related research which utilizes nanomaterials and nanotechnology. Manuscripts of four types are considered: review articles which inform readers of the latest research and advances in energy science; rapid communications which feature exciting research breakthroughs in the field; full-length articles which report comprehensive research developments; and news and opinions which comment on topical issues or express views on the developments in related fields.
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