Experimental investigation of bed-to-wall heat transfer in fluidized beds of a Geldart B sorbent particle under a full spectrum of fluidization regime

IF 4.1 2区 材料科学 Q2 ENGINEERING, CHEMICAL Particuology Pub Date : 2024-07-10 DOI:10.1016/j.partic.2024.07.001
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Abstract

Fluidization technology has been used in CO2 capture processes, the successful design and operation of the heat exchangers involved in this process require much information on the bed-to-wall heat transfer of the sorbent particles in fluidized states. In this study, the bed-to-wall heat transfer coefficient (h) of a solid amine sorbent was measured by a heat transfer probe in a large-scale circulating fluidized bed cold model unit, where full spectrum of fluidization regimes can be realized. The corresponding hydrodynamic signals were also studied by pressure sensors and optical fiber probes to further explain the newly discovered phenomenon. The results show that in a dense bed, due to the counterbalanced effect of time fraction of packet and packet renewal frequency, h of the Geldart B particle reaches a peak within the bubbling fluidized regime, and the radial distribution of h are opposite in bubbling and turbulent fluidized regimes. In a fast fluidization regime, gas convection becomes the dominant factor affecting h when the solids holdup is low enough. Correlations were provided or recommended to guide the design of heat exchangers in the fluidized bed CO2 capture processes.

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流化床中 Geldart B 吸附颗粒在全谱流化条件下的床壁传热实验研究
流化技术已被应用于二氧化碳捕集工艺中,该工艺中热交换器的成功设计和运行需要大量有关流化状态下吸附剂颗粒床壁传热的信息。本研究在大型循环流化床冷模型装置中使用传热探头测量了固体胺吸附剂的床壁传热系数(h),该装置可实现全流化状态。此外,还通过压力传感器和光纤探头研究了相应的流体动力信号,以进一步解释新发现的现象。结果表明,在稠密床层中,由于气包时间分数和气包更新频率的平衡作用,Geldart B 粒子的 h 值在气泡流化体系中达到峰值,而 h 值的径向分布在气泡流化体系和湍流流化体系中是相反的。在快速流化体系中,当固体截留率足够低时,气体对流成为影响 h 的主要因素。为指导流化床二氧化碳捕集过程中热交换器的设计,提供或建议了相关性。
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来源期刊
Particuology
Particuology 工程技术-材料科学:综合
CiteScore
6.70
自引率
2.90%
发文量
1730
审稿时长
32 days
期刊介绍: The word ‘particuology’ was coined to parallel the discipline for the science and technology of particles. Particuology is an interdisciplinary journal that publishes frontier research articles and critical reviews on the discovery, formulation and engineering of particulate materials, processes and systems. It especially welcomes contributions utilising advanced theoretical, modelling and measurement methods to enable the discovery and creation of new particulate materials, and the manufacturing of functional particulate-based products, such as sensors. Papers are handled by Thematic Editors who oversee contributions from specific subject fields. These fields are classified into: Particle Synthesis and Modification; Particle Characterization and Measurement; Granular Systems and Bulk Solids Technology; Fluidization and Particle-Fluid Systems; Aerosols; and Applications of Particle Technology. Key topics concerning the creation and processing of particulates include: -Modelling and simulation of particle formation, collective behaviour of particles and systems for particle production over a broad spectrum of length scales -Mining of experimental data for particle synthesis and surface properties to facilitate the creation of new materials and processes -Particle design and preparation including controlled response and sensing functionalities in formation, delivery systems and biological systems, etc. -Experimental and computational methods for visualization and analysis of particulate system. These topics are broadly relevant to the production of materials, pharmaceuticals and food, and to the conversion of energy resources to fuels and protection of the environment.
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