Hydrogel polymer electrolytes toward better zinc-ion batteries: A comprehensive review

IF 36.6 Q1 ELECTROCHEMISTRY eScience Pub Date : 2025-03-01 Epub Date: 2024-07-09 DOI:10.1016/j.esci.2024.100294
Jianwen Li , Alireza Azizi , Shuang Zhou , Sainan Liu , Chao Han , Zhi Chang , Anqiang Pan , Guozhong Cao
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Abstract

Aqueous zinc-ion batteries (ZIBs) represent a promising solution for “beyond-lithium-ion” chemistries, but certain problems hinder their further development, especially when conventional aqueous electrolytes are involved. Hydrogel polymer electrolytes (HPEs) offer opportunities to circumvent these issues. This review aims to provide a fundamental understanding of how to design better HPEs for high-performing ZIBs, through critically analyzing the recent literature. Concerns regarding HPEs’ mechanical, interfacial, and electrochemical characteristics are addressed, followed by in-depth insights into their underlying mechanisms. Possibilities for practical applications of HPEs are also discussed.

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水凝胶聚合物电解质用于制造更好的锌离子电池:综述
水锌离子电池(zib)代表了一种很有前途的“超越锂离子”化学解决方案,但某些问题阻碍了它们的进一步发展,特别是当涉及到传统的水电解质时。水凝胶聚合物电解质(HPEs)提供了避免这些问题的机会。本综述旨在通过批判性地分析最近的文献,为如何为高性能zib设计更好的hpe提供基本的理解。对HPEs的机械、界面和电化学特性进行了讨论,然后深入了解了其潜在机制。讨论了hpe实际应用的可能性。
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33.70
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