Thermoelectric transport and current noise through a multilevel Anderson impurity: Three-body Fermi liquid corrections in quantum dots and magnetic alloys

IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Physical Review B Pub Date : 2024-07-23 DOI:10.1103/physrevb.110.035308
Yoshimichi Teratani, Kazuhiko Tsutsumi, Kaiji Motoyama, Rui Sakano, Akira Oguri
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Our formulation for the low-energy transport is based on an Anderson model with <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>N</mi></math> discrete impurity levels, and is asymptotically exact at low energies, up to the next-leading order terms in power expansions with respect to temperature <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>T</mi></math> and bias voltage <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><mi>e</mi><mi>V</mi></mrow></math>. The expansion coefficients can be expressed in terms of the Fermi liquid parameters, which include the three-body correlation functions defined with respect to the equilibrium ground state in addition to the linear susceptibilities and the occupation number <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><msubsup><mi>N</mi><mi>d</mi><mrow></mrow></msubsup></math> of impurity electrons. We apply this formulation to the <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><mi>SU</mi><mo>(</mo><mi>N</mi><mo>)</mo></mrow></math> symmetric QD and MA, and calculate the correlation functions for <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><mi>N</mi><mo>=</mo><mn>4</mn></mrow></math> and 6, using numerical renormalization group approach. The three-body correlations are shown to be determined by a single parameter over a wide range of electron fillings <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><mn>1</mn><mo>≲</mo><msubsup><mi>N</mi><mi>d</mi><mrow></mrow></msubsup><mo>≲</mo><mi>N</mi><mo>−</mo><mn>1</mn></mrow></math> for strong Coulomb interactions <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>U</mi></math>, and they also exhibit the plateau structures due to the <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><mi>SU</mi><mo>(</mo><mi>N</mi><mo>)</mo></mrow></math> Kondo effects at integer values of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><msubsup><mi>N</mi><mi>d</mi><mrow></mrow></msubsup></math>. 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Furthermore, we find that the current noise for the SU(4) quantum dots and that for SU(6) show a pronounced difference at the quarter <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msubsup><mi>N</mi><mi>d</mi><mrow></mrow></msubsup><mo>/</mo><mi>N</mi><mo>=</mo><mn>1</mn><mo>/</mo><mn>4</mn></mrow></math> and <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><mn>3</mn><mo>/</mo><mn>4</mn></mrow></math> fillings. 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Abstract

We present a comprehensive Fermi liquid description for thermoelectric transport and current noise, applicable to multilevel quantum dots (QD) and magnetic alloys (MA) without electron-hole or time-reversal symmetry. Our formulation for the low-energy transport is based on an Anderson model with N discrete impurity levels, and is asymptotically exact at low energies, up to the next-leading order terms in power expansions with respect to temperature T and bias voltage eV. The expansion coefficients can be expressed in terms of the Fermi liquid parameters, which include the three-body correlation functions defined with respect to the equilibrium ground state in addition to the linear susceptibilities and the occupation number Nd of impurity electrons. We apply this formulation to the SU(N) symmetric QD and MA, and calculate the correlation functions for N=4 and 6, using numerical renormalization group approach. The three-body correlations are shown to be determined by a single parameter over a wide range of electron fillings 1NdN1 for strong Coulomb interactions U, and they also exhibit the plateau structures due to the SU(N) Kondo effects at integer values of Nd. We find that the Lorenz number L=κ/(Tσ) for QD and MA, defined as the ratio of the thermal conductivity κ to the electrical conductivity σ, deviates from the universal Wiedemann-Franz value π2/(3e2) as the temperature increases from T=0, showing the T2 dependence, the coefficient for which depends on the three-body correlations away from half filling. Furthermore, we find that the current noise for the SU(4) quantum dots and that for SU(6) show a pronounced difference at the quarter Nd/N=1/4 and 3/4 fillings. In particular, the linear noise for N=4 exhibits a flat peak while the peak for N=6 shows a round shape, reflecting the fact that, at these filling points, the SU(N) Kondo effects occur for N0 (mod 4), whereas the intermediate-valence fluctuations occur for N2 (mod 4). We also demonstrate the role of three-body correlations on the nonlinear current noise and the other transport coefficients.

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通过多级安德森杂质的热电传输和电流噪声:量子点和磁性合金中的三体费米液体校正
我们提出了热电输运和电流噪声的费米液体综合描述,适用于无电子-空穴或时间反转对称性的多级量子点(QD)和磁性合金(MA)。我们的低能输运公式基于具有 N 个离散杂质级的安德森模型,在低能时近似精确,直到与温度 T 和偏置电压 eV 有关的幂级数展开的下一阶项。膨胀系数可以用费米液体参数来表示,其中除了线性感性和杂质电子的占据数 Nd 外,还包括针对平衡基态定义的三体相关函数。我们将这一公式应用于苏(N)对称 QD 和 MA,并利用数值重正化群方法计算了 N=4 和 6 的相关函数。结果表明,在强库仑相互作用 U 下,三体相关函数在电子填充 1≲Nd≲N-1 的宽范围内由单一参数决定,而且在 Nd 的整数值时,它们还表现出 SU(N) Kondo 效应导致的高原结构。我们发现,QD 和 MA 的洛伦兹数 L=κ/(Tσ) 定义为热导率 κ 与电导率 σ 之比,随着温度从 T=0 升高,洛伦兹数偏离了通用的维德曼-弗朗茨值 π2/(3e2),显示出与 T2 有关,其系数取决于远离半填充的三体相关性。此外,我们发现 SU(4) 量子点的电流噪声和 SU(6) 量子点的电流噪声在四分之一 Nd/N=1/4 和 3/4 填充时有明显差异。特别是,N=4 的线性噪声表现出一个平坦的峰值,而 N=6 的峰值则表现出一个圆形,这反映出在这些填充点,SU(N) Kondo 效应发生在 N≡0 (mod 4),而中间价波动发生在 N≡2 (mod 4)。我们还证明了三体关联对非线性电流噪声和其他输运系数的作用。
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来源期刊
Physical Review B
Physical Review B 物理-物理:凝聚态物理
CiteScore
6.70
自引率
32.40%
发文量
0
审稿时长
3.0 months
期刊介绍: Physical Review B (PRB) is the world’s largest dedicated physics journal, publishing approximately 100 new, high-quality papers each week. The most highly cited journal in condensed matter physics, PRB provides outstanding depth and breadth of coverage, combined with unrivaled context and background for ongoing research by scientists worldwide. PRB covers the full range of condensed matter, materials physics, and related subfields, including: -Structure and phase transitions -Ferroelectrics and multiferroics -Disordered systems and alloys -Magnetism -Superconductivity -Electronic structure, photonics, and metamaterials -Semiconductors and mesoscopic systems -Surfaces, nanoscience, and two-dimensional materials -Topological states of matter
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