Remagnetization kinetics of soft ferrogels

A. Yu. Zubarev, L. Yu. Iskakova
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Abstract

We present the results of the theoretical analysis of remagnetization kinetics and magnetic hyperthermia effect in a single-domain ferromagnetic particle embedded in a soft elastic-viscous medium (gel or biological tissue for example). Unlike previous studies, we consider simultaneous action of both main mechanisms of particle remagnetization in an alternating magnetic field. Namely, (i) its body turn (rotation) with its magnetic moment and (ii) the Neel remagnetization through the potential barrier of the particle magnetic anisotropy. We suppose that the energy of the particle Zeeman interaction with the field is less than the energy of the anisotropy; no other restrictions on the field strength are assumed. In the linear, with respect to this field, approximation, the frequency dependences of the real and imaginary parts of the particle complex susceptibility are calculated in more details. The real part monotonic decreases with the field frequency. If the host medium is rigid enough, the imaginary part of the susceptibility has a maximum, corresponding to the Neel relaxation. In the soft system, it has maximum, reflecting the particle rotation in the field. In the intermediate case, our calculations demonstrate two maximums of the imaginary part. We hope the present results will be useful for the development of scientific basement of magnetic hyperthermia therapy of oncological diseases.

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软铁凝胶的再磁化动力学
我们介绍了嵌入软弹性粘性介质(例如凝胶或生物组织)中的单域铁磁粒子的再磁化动力学和磁热效应的理论分析结果。与以往的研究不同,我们考虑了交变磁场中粒子再磁化的两种主要机制的同时作用。即:(i) 粒子磁矩的体转(旋转);(ii) 通过粒子磁各向异性势垒的 Neel 再磁化。我们假设粒子与磁场的泽曼相互作用的能量小于各向异性的能量;对磁场强度没有其他限制。在与该场有关的线性近似中,我们更详细地计算了粒子复感性实部和虚部的频率依赖性。实部随场频率单调递减。如果主介质足够坚硬,则电感的虚部会达到最大值,与尼尔弛豫相对应。在软系统中,它有一个最大值,反映了粒子在磁场中的旋转。在中间情况下,我们的计算显示了两个虚部最大值。我们希望目前的结果将有助于开发磁热疗法治疗肿瘤疾病的科学基础。
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