Layered double hydroxides and metal-organic frameworks for electrocatalytic CO2 reduction: A comprehensive review

IF 3.1 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Carbon Trends Pub Date : 2024-07-22 DOI:10.1016/j.cartre.2024.100384

Mahider Asmare Tekalgne , Ha Huu Do , Gyeong Ho Han , Sung Hyun Hong , Jin Hyuk Cho , Sang Hyun Ahn , Soo Young Kim

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Abstract

Electrocatalytic carbon dioxide (CO₂) reduction has emerged as a promising approach for converting CO₂ into value-added products and mitigating greenhouse gas emissions. Layered double hydroxides (LDHs) and metal-organic frameworks (MOFs) have attracted significant attention as potential electrocatalysts for CO₂ reduction due to their unique structural properties and tunable chemical compositions. In this review, we provide a comprehensive overview of recent advances in the utilization of LDHs and MOFs as electrocatalysts for CO₂ reduction. Scrutiny on various catalysts, along with their general design ways for CO₂ reduction is presented. This review will provide insight into the up-to-date research progress in MOF-based materials for CO₂ conversion. Furthermore, we highlight opportunities in this field and propose future research directions aimed at optimizing the performance of LDHs and MOFs for CO₂ reduction applications.

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用于电催化二氧化碳还原的层状双氢氧化物和金属有机框架：全面综述

电催化二氧化碳（CO2）还原已成为将二氧化碳转化为高附加值产品和减少温室气体排放的一种前景广阔的方法。层状双氢氧化物（LDHs）和金属有机框架（MOFs）作为潜在的二氧化碳还原电催化剂，因其独特的结构特性和可调整的化学成分而备受关注。在本综述中，我们将全面概述利用 LDHs 和 MOFs 作为二氧化碳还原电催化剂的最新进展。文中介绍了各种催化剂及其用于二氧化碳还原的一般设计方法。本综述将深入介绍基于 MOF 的二氧化碳转化材料的最新研究进展。此外，我们还强调了这一领域的机遇，并提出了未来的研究方向，旨在优化 LDHs 和 MOFs 在二氧化碳还原应用中的性能。

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