One-step solvothermal synthesis of Zn2SnO4/rGO composite material and highly gas sensing performance to acetone

IF 3.4 3区 化学 Q2 CHEMISTRY, INORGANIC & NUCLEAR Solid State Sciences Pub Date : 2024-07-26 DOI:10.1016/j.solidstatesciences.2024.107638
Fang He , Qimeng Du , Yulong Zhang , Wenxin Gao , Hang Chen , Chunxu Wang , Dekuan Liu , Yaomin Zhao , Tiebing Cui , Qi Qin
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Abstract

In this study, one-step solvothermal method was employed to synthesize Zn2SnO4 and Zn2SnO4/rGO composites. Zn2SnO4 was bonded to the rGO surface or in the spaces between the lamellar layers to create a semiconductor composite material that is physically supported by heterojunction. Compared to Zn2SnO4 sensor, the Zn2SnO4/rGO sensing material exhibits superior gas-sensing properties to acetone. The optimal temperature of Zn2SnO4/rGO sensor was just 200 °C, while its sensitivity to 100 ppm acetone gas was up to 11.2. Its response and recovery times were only 8 s and 11 s, respectively. The large specific surface area and distinctive heterojunction of the composite material are responsible for the enhanced gas-sensing performance of Zn2SnO4/rGO sensing material. Zn2SnO4/rGO is an ideal sensing material due to high sensitivity, fast response/recovery properties, great selectivity, and stability.

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一步溶热合成 Zn2SnO4/rGO 复合材料及其对丙酮的高气体传感性能
本研究采用一步溶热法合成 ZnSnO 和 ZnSnO/rGO 复合材料。ZnSnO 被键合在 rGO 表面或薄片层之间的空隙中,形成了一种异质结物理支撑的半导体复合材料。与 ZnSnO 传感器相比,ZnSnO/rGO 传感材料对丙酮的气体传感性能更优越。ZnSnO/rGO 传感器的最佳温度仅为 200 ℃,而其对 100 ppm 丙酮气体的灵敏度高达 11.2。其响应时间和恢复时间分别仅为 8 秒和 11 秒。复合材料的大比表面积和独特的异质结是 ZnSnO/rGO 传感材料气体传感性能增强的原因。ZnSnO/rGO 具有高灵敏度、快速响应/恢复特性、高选择性和稳定性,是一种理想的传感材料。
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来源期刊
Solid State Sciences
Solid State Sciences 化学-无机化学与核化学
CiteScore
6.60
自引率
2.90%
发文量
214
审稿时长
27 days
期刊介绍: Solid State Sciences is the journal for researchers from the broad solid state chemistry and physics community. It publishes key articles on all aspects of solid state synthesis, structure-property relationships, theory and functionalities, in relation with experiments. Key topics for stand-alone papers and special issues: -Novel ways of synthesis, inorganic functional materials, including porous and glassy materials, hybrid organic-inorganic compounds and nanomaterials -Physical properties, emphasizing but not limited to the electrical, magnetical and optical features -Materials related to information technology and energy and environmental sciences. The journal publishes feature articles from experts in the field upon invitation. Solid State Sciences - your gateway to energy-related materials.
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