Lattice dynamics of119Sn impurity in a bcc-Cr crystal.

IF 2.3 4区 物理与天体物理 Q3 PHYSICS, CONDENSED MATTER Journal of Physics: Condensed Matter Pub Date : 2024-08-23 DOI:10.1088/1361-648X/ad6c97
Stanisław M Dubiel, Michael Y Hu, Małgorzata Sternik, E Ercan Alp, Ahmet Alatas, Ayman Said, Krzysztof Parlinski, Przemysław Piekarz
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Abstract

The chromium crystal doped with119Sn isotope was studied using the nuclear resonance inelastic x-ray scattering and first principles calculations. The Sn partial phonon density of states (PDOS) was obtained for three temperatures that correspond to different magnetic states of Cr. At all temperatures, the energy spectrum consists of a broad band around 18 meV and a narrow peak at 43 meV. The additional peak around 39 meV is observed only in the magnetically ordered phases, indicating the influence of magnetic order in chromium on lattice dynamics. The partial PDOS calculated with the antiferromagnetic order on Cr atoms show a very good agreement with the experimental data. It is revealed that the high-energy peak is lying above the phonon spectra of the pure bcc-Cr crystal. These are the local modes with the increased energies due to a strongly reduced distance between Sn and the nearest-neighbor Cr atoms.

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bcc-Cr 晶体中 119Sn 杂质的晶格动力学。
利用核共振非弹性 X 射线散射和第一原理计算,研究了掺杂 119 Sn 同位素的铬晶体。获得了与铬的不同磁态相对应的三个温度下的锡部分声子状态密度。在所有温度下,能谱由 18 meV 附近的宽带和 43 meV 处的窄峰组成。只有在磁有序相中才能观察到 39 meV 附近的附加峰值,这表明铬的磁有序性对晶格动力学有影响。根据铬原子上的反铁磁有序性计算出的部分声子 态密度与实验数据非常吻合。研究发现,高能峰位于纯 bcc-Cr 晶体声子谱的上方。这些是局部模式 ,由于锡和最近邻近的铬原子之间的距离大大缩短,导致能量增加。
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来源期刊
Journal of Physics: Condensed Matter
Journal of Physics: Condensed Matter 物理-物理:凝聚态物理
CiteScore
5.30
自引率
7.40%
发文量
1288
审稿时长
2.1 months
期刊介绍: Journal of Physics: Condensed Matter covers the whole of condensed matter physics including soft condensed matter and nanostructures. Papers may report experimental, theoretical and simulation studies. Note that papers must contain fundamental condensed matter science: papers reporting methods of materials preparation or properties of materials without novel condensed matter content will not be accepted.
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