Multifunctional performances of structural battery composite full-cells based on carbon fiber anode and LiFePO4 loaded carbon fiber cathode

IF 5 2区 材料科学 Q1 MATERIALS SCIENCE, CHARACTERIZATION & TESTING Polymer Testing Pub Date : 2024-08-01 DOI:10.1016/j.polymertesting.2024.108523
Guocheng Qi , Yunlong Wu , Yinghui Ding , Boming Zhang
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Abstract

In this work, the structural battery composite (SBC) full-cells based on carbon fiber (CFs) were fabricated using a three-step hot pressing method. LiFePO4 (LFP) was loaded onto CF fabrics considering the influences of hot pressing parameters including the pressure and the temperature. The SBC full-cells were subsequently fabricated using the LFP loaded CF cathode, the CF anode, the glass fiber (GF) separator via a structural electrolyte (SE) filming process, followed by the second hot pressing. The multifunctional efficiencies were assessed for SBCs with SE containing different components. To reduce the capacity loss, the SBC was eventually encapsulated with the GF/Vinyl Ester prepreg and thermally cured in the third hot pressing. The capacity retention of the SBC was significantly improved after encapsulation. This work could be seen as a further step forward the engineering fabrication of the SBC full-cells based on both CF anodes and cathodes.

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基于碳纤维阳极和负载磷酸铁锂的碳纤维阴极的全电池结构复合材料的多功能性能
本研究采用三步热压法制造了基于碳纤维(CF)的结构电池复合材料(SBC)全电池。考虑到热压参数(包括压力和温度)的影响,将磷酸铁锂(LFP)负载到碳纤维织物上。随后,通过结构电解质(SE)薄膜工艺,使用装载了 LFP 的 CF 阴极、CF 阳极和玻璃纤维(GF)隔膜制造出 SBC 全电池,然后进行第二次热压。对含有不同成分 SE 的 SBC 的多功能效率进行了评估。为减少容量损失,SBC 最终采用 GF/乙烯基酯预浸料封装,并在第三次热压中进行热固化。封装后,SBC 的容量保持率明显提高。这项工作可视为在基于 CF 阳极和阴极的 SBC 全电池工程制造方面又向前迈进了一步。
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来源期刊
Polymer Testing
Polymer Testing 工程技术-材料科学:表征与测试
CiteScore
10.70
自引率
5.90%
发文量
328
审稿时长
44 days
期刊介绍: Polymer Testing focuses on the testing, analysis and characterization of polymer materials, including both synthetic and natural or biobased polymers. Novel testing methods and the testing of novel polymeric materials in bulk, solution and dispersion is covered. In addition, we welcome the submission of the testing of polymeric materials for a wide range of applications and industrial products as well as nanoscale characterization. The scope includes but is not limited to the following main topics: Novel testing methods and Chemical analysis • mechanical, thermal, electrical, chemical, imaging, spectroscopy, scattering and rheology Physical properties and behaviour of novel polymer systems • nanoscale properties, morphology, transport properties Degradation and recycling of polymeric materials when combined with novel testing or characterization methods • degradation, biodegradation, ageing and fire retardancy Modelling and Simulation work will be only considered when it is linked to new or previously published experimental results.
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