Graphitic carbon nitride(g-C3N4)-based photocatalysts for dye removal: Current status

Dhruti Sundar Pattanayak , Madhu Surana , Aditya Kumar , Dhananjay Singh , Dharm Pal
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Abstract

Water contamination is a global concern as a result of growing industrialization and urbanization. Dye waste produced by numerous industries pollutes the water, so dye-based wastewater is a major alarm for animals, human health, and the environment. The elimination of these dye contaminants from water supplies is currently critical and significant due to the dyes' toxicity on humans, livestock, and plants. To remove/degrade dyes, various methods have been investigated, including extraction, absorption, membrane separation, coagulation, adsorption, biological treatment, and advanced oxidation process (AOPs). Graphitic carbon nitride (g-C3N4), a captivating formed polymer, has been transformed as an intriguing issue in AOP science because of its metal-free advantages and its high sensitivity to light. Accordingly, when AOPs are joined with g-C3N4, superb dye degradation has occurred. This paper overviewed the g-C3N4-based AOPs are discussed for dye removal. The synergist effectiveness and mechanisms behind catalytic activity of g-C3N4-based catalysts are broadly discussed. In the meantime, the impacts of pH, water temperature, dissolved oxygen, initial dye concentration, catalyst dosage, and scavengers on the reaction carried out by g-C3N4-based catalysts are illustrated.

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基于石墨氮化碳(g-C3N4)的用于去除染料的光催化剂:现状
随着工业化和城市化的发展,水污染已成为全球关注的问题。众多行业产生的染料废水污染了水源,因此染料废水对动物、人类健康和环境都是一个重大警报。由于染料对人类、牲畜和植物的毒性,目前从供水中消除这些染料污染物至关重要,意义重大。为了去除/降解染料,人们研究了各种方法,包括萃取、吸收、膜分离、混凝、吸附、生物处理和高级氧化工艺(AOPs)。氮化石墨碳(g-C3N4)是一种迷人的成型聚合物,因其不含金属的优点和对光的高灵敏度,已成为 AOP 科学中一个引人关注的问题。因此,当 AOP 与 g-C3N4 结合使用时,会产生极佳的染料降解效果。本文概述了基于 g-C3N4 的 AOPs 在染料去除方面的应用。对 g-C3N4 基催化剂的增效作用及其催化活性的机理进行了广泛的讨论。同时,阐述了 pH 值、水温、溶解氧、初始染料浓度、催化剂用量和清除剂对 g-C3N4 基催化剂反应的影响。
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