Hanbin Deng, Hailang Qin, Guowei Liu, Tianyu Yang, Ruiqing Fu, Zhongyi Zhang, Xianxin Wu, Zhiwei Wang, Youguo Shi, Jinjin Liu, Hongxiong Liu, Xiao-Yu Yan, Wei Song, Xitong Xu, Yuanyuan Zhao, Mingsheng Yi, Gang Xu, Hendrik Hohmann, Sofie Castro Holbæk, Matteo Dürrnagel, Sen Zhou, Guoqing Chang, Yugui Yao, Qianghua Wang, Zurab Guguchia, Titus Neupert, Ronny Thomale, Mark H. Fischer, Jia-Xin Yin
{"title":"Chiral kagome superconductivity modulations with residual Fermi arcs","authors":"Hanbin Deng, Hailang Qin, Guowei Liu, Tianyu Yang, Ruiqing Fu, Zhongyi Zhang, Xianxin Wu, Zhiwei Wang, Youguo Shi, Jinjin Liu, Hongxiong Liu, Xiao-Yu Yan, Wei Song, Xitong Xu, Yuanyuan Zhao, Mingsheng Yi, Gang Xu, Hendrik Hohmann, Sofie Castro Holbæk, Matteo Dürrnagel, Sen Zhou, Guoqing Chang, Yugui Yao, Qianghua Wang, Zurab Guguchia, Titus Neupert, Ronny Thomale, Mark H. Fischer, Jia-Xin Yin","doi":"10.1038/s41586-024-07798-y","DOIUrl":null,"url":null,"abstract":"Superconductivity involving finite-momentum pairing1 can lead to spatial-gap and pair-density modulations, as well as Bogoliubov Fermi states within the superconducting gap. However, the experimental realization of their intertwined relations has been challenging. Here we detect chiral kagome superconductivity modulations with residual Fermi arcs in KV3Sb5 and CsV3Sb5 using normal and Josephson scanning tunnelling microscopy down to 30 millikelvin with a resolved electronic energy difference at the microelectronvolt level. We observe a U-shaped superconducting gap with flat residual in-gap states. This gap shows chiral 2a × 2a spatial modulations with magnetic-field-tunable chirality, which align with the chiral 2a × 2a pair-density modulations observed through Josephson tunnelling. These findings demonstrate a chiral pair density wave (PDW) that breaks time-reversal symmetry. Quasiparticle interference imaging of the in-gap zero-energy states reveals segmented arcs, with high-temperature data linking them to parts of the reconstructed vanadium d-orbital states within the charge order. The detected residual Fermi arcs can be explained by the partial suppression of these d-orbital states through an interorbital 2a × 2a PDW and thus serve as candidate Bogoliubov Fermi states. In addition, we differentiate the observed PDW order from impurity-induced gap modulations. Our observations not only uncover a chiral PDW order with orbital selectivity but also show the fundamental space–momentum correspondence inherent in finite-momentum-paired superconductivity. Using normal and Josephson scanning tunnelling microscopy, chiral kagome superconductivity modulations with corresponding residual Fermi arcs are detected in KV3Sb5 and CsV3Sb5.","PeriodicalId":18787,"journal":{"name":"Nature","volume":null,"pages":null},"PeriodicalIF":50.5000,"publicationDate":"2024-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature","FirstCategoryId":"103","ListUrlMain":"https://www.nature.com/articles/s41586-024-07798-y","RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MULTIDISCIPLINARY SCIENCES","Score":null,"Total":0}
引用次数: 0
Abstract
Superconductivity involving finite-momentum pairing1 can lead to spatial-gap and pair-density modulations, as well as Bogoliubov Fermi states within the superconducting gap. However, the experimental realization of their intertwined relations has been challenging. Here we detect chiral kagome superconductivity modulations with residual Fermi arcs in KV3Sb5 and CsV3Sb5 using normal and Josephson scanning tunnelling microscopy down to 30 millikelvin with a resolved electronic energy difference at the microelectronvolt level. We observe a U-shaped superconducting gap with flat residual in-gap states. This gap shows chiral 2a × 2a spatial modulations with magnetic-field-tunable chirality, which align with the chiral 2a × 2a pair-density modulations observed through Josephson tunnelling. These findings demonstrate a chiral pair density wave (PDW) that breaks time-reversal symmetry. Quasiparticle interference imaging of the in-gap zero-energy states reveals segmented arcs, with high-temperature data linking them to parts of the reconstructed vanadium d-orbital states within the charge order. The detected residual Fermi arcs can be explained by the partial suppression of these d-orbital states through an interorbital 2a × 2a PDW and thus serve as candidate Bogoliubov Fermi states. In addition, we differentiate the observed PDW order from impurity-induced gap modulations. Our observations not only uncover a chiral PDW order with orbital selectivity but also show the fundamental space–momentum correspondence inherent in finite-momentum-paired superconductivity. Using normal and Josephson scanning tunnelling microscopy, chiral kagome superconductivity modulations with corresponding residual Fermi arcs are detected in KV3Sb5 and CsV3Sb5.
期刊介绍:
Nature is a prestigious international journal that publishes peer-reviewed research in various scientific and technological fields. The selection of articles is based on criteria such as originality, importance, interdisciplinary relevance, timeliness, accessibility, elegance, and surprising conclusions. In addition to showcasing significant scientific advances, Nature delivers rapid, authoritative, insightful news, and interpretation of current and upcoming trends impacting science, scientists, and the broader public. The journal serves a dual purpose: firstly, to promptly share noteworthy scientific advances and foster discussions among scientists, and secondly, to ensure the swift dissemination of scientific results globally, emphasizing their significance for knowledge, culture, and daily life.