Mobile laboratory measurements of air pollutants in Baltimore, MD elucidate issues of environmental justice.

IF 4.6 Q2 MATERIALS SCIENCE, BIOMATERIALS ACS Applied Bio Materials Pub Date : 2024-11-01 Epub Date: 2024-09-16 DOI:10.1080/10962247.2024.2393178
Russell R Dickerson, Phillip Stratton, Xinrong Ren, Paul Kelley, Christopher D Heaney, Lauren Deanes, Matthew Aubourg, Kristoffer Spicer, Joel Dreessen, Ryan Auvil, Gregory Sawtell, Meleny Thomas, Shashawnda Campbell, Carlos Sanchez
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Abstract

The City of Baltimore, MD has a history of problems with environmental justice (EJ), air pollution, and the urban heat island (UHI) effect. Current chemical transport models lack the resolution to simulate concentrations on the scale needed, about 100 m, to identify the neighborhoods with anomalously high air pollution levels. In this paper we introduce the capabilities of a mobile laboratory and an initial survey of several pollutants in Baltimore to identify which communities are exposed to disproportionate concentrations of air pollution and to which species. High concentrations of black carbon (BC) stood out at some locations - near major highways, downtown, and in the Curtis Bay neighborhood of Baltimore. Results from the mobile lab are confirmed with longer-term, low-cost monitoring. In Curtis Bay, higher concentrations of BC were measured along Pennington Ave. (mean [5th to 95th percentiles] = 2.08 [2.0-10.9] μg m-3) than along Curtis Ave. just ~ 150 m away (0.67[0.1 - 1.8] μg m-3). Other species, including criteria pollutants ozone (O3), carbon monoxide (CO), nitrogen dioxide (NO2), sulfur dioxide (SO2), and fine particulate matter (PM2.5), showed little gradient. Observations with high spatial and temporal resolution help isolate the mechanisms leading to locally high pollutant concentrations. The difference in BC appears to result not from heavier truck traffic or slower dispersion but from the interruptions in traffic flow. Pennington Ave. has three stoplights while Curtis Ave. has none. As heavy-duty diesel-powered vehicles accelerate, they experience turbo-lag and the resulting rich air-fuel mixture exacerbates BC emissions. Immediate mediation might be achieved through smoother traffic flow, and the long-term solution through replacing heavy-duty trucks with electric vehicles.Implications: We present results documenting the locations within Baltimore of high concentrations of Black Carbon pollution and identify the likely source - diesel exhaust emissions exacerbated by stop-and-go traffic and associated turbo-lag. This suggests solutions (smoother traffic, retrofit particulate filters, replacement of diesel with electric vehicles) that would enhance Environmental Justice (EJ) and could be applied to other cities with EJ problems.Synopsis: This paper presents observations of atmospheric black carbon aerosol showing impacts on environmental justice, then identifies causes and suggests solutions.

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对马里兰州巴尔的摩市空气污染物的移动实验室测量阐明了环境正义问题。
马里兰州巴尔的摩市历来存在环境正义 (EJ)、空气污染和城市热岛 (UHI) 效应等问题。目前的化学传输模型缺乏分辨率,无法模拟约 100 米范围内的浓度,因此无法确定空气污染水平异常高的街区。在本文中,我们介绍了移动实验室的功能,并对巴尔的摩的几种污染物进行了初步调查,以确定哪些社区暴露于不成比例的空气污染浓度中,以及哪些污染物的种类。黑碳 (BC) 的高浓度在巴尔的摩的主要高速公路附近、市中心和柯蒂斯湾社区等地尤为突出。移动实验室的结果得到了长期、低成本监测的证实。在 Curtis Bay,沿 Pennington 大道测得的 BC 浓度(平均值 [第 5 到第 95 百分位数] = 2.08 [2.0- 10.9] μg m-3)高于仅相距约 150 米的 Curtis 大道(0.67 [0.1- 1.8] μg m-3)。其他物种,包括标准污染物臭氧 (O3)、一氧化碳 (CO)、二氧化氮 (NO2)、二氧化硫 (SO2) 和细颗粒物 (PM2.5),几乎没有显示出梯度。高空间和时间分辨率的观测有助于分离出导致局部污染物高浓度的机制。BC 的差异似乎不是由于卡车交通量较大或扩散速度较慢,而是由于交通流的中断。彭宁顿大道有三个红绿灯,而柯蒂斯大道则没有。重型柴油发动机车辆在加速时会出现涡轮滞后现象,由此产生的高浓度空气-燃料混合物会加剧 BC 排放。近期可通过更顺畅的交通流进行调解,而长期解决方案则是用电动汽车取代重型卡车:我们的研究结果记录了巴尔的摩市内黑碳污染浓度较高的地点,并确定了可能的来源--柴油尾气排放因走走停停的交通和相关涡轮滞后而加剧。这就提出了解决方案(更顺畅的交通、改装微粒过滤器、用电动车取代柴油车),这些方案将加强环境正义(EJ),并可应用于存在环境正义问题的其他城市。简要说明:本文介绍了大气黑碳气溶胶的观测结果,显示了对环境正义的影响,然后找出了原因并提出了解决方案。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
ACS Applied Bio Materials
ACS Applied Bio Materials Chemistry-Chemistry (all)
CiteScore
9.40
自引率
2.10%
发文量
464
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