Integrating direct air capture with algal biofuel production to reduce cost, energy, and GHG emissions

IF 7.2 2区 工程技术 Q1 CHEMISTRY, MULTIDISCIPLINARY Journal of CO2 Utilization Pub Date : 2024-08-01 DOI:10.1016/j.jcou.2024.102911
S. D’Souza , J. Johnston , V.M. Thomas , K. Harris , E.C.D. Tan , R.R. Chance , Y. Yuan
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Abstract

We investigate the potential to reduce costs and greenhouse gas emissions of the utilization of direct air capture of CO2 (DAC) for the production of algal biofuel. We examine four integrated designs for a DAC system comprised of solid amine monolith adsorbents delivering CO2 at the required level for algae cultivation with a photobioreactor (PBR)-based fuel production facility. We show that the integration of DAC with this biofuel production facility provides cost and greenhouse gas emissions benefits. Heat integration decreases operating expenses by reducing energy demand for heating requirements. Mass integration, utilizing flue gas CO2 as a carbon source for the PBRs, decreases the DAC system scale, resulting in both capital and operating cost savings. The most advantageous option depends on the interplay of heat and mass integration while matching the diurnal rhythm of algal growth with the inherently steady pace and energy requirements of the DAC system and fuel production. For these technologies, the DAC-PBR mass and energy integration provides an 18 % cost reduction and a 50 % reduction in greenhouse gas emissions for the current state of the technology.

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将直接空气捕集与藻类生物燃料生产相结合,以降低成本、能源和温室气体排放
我们研究了利用直接空气捕集二氧化碳(DAC)生产藻类生物燃料降低成本和减少温室气体排放的潜力。我们研究了由固体胺整体吸附剂组成的 DAC 系统的四种集成设计,该系统通过基于光生物反应器 (PBR) 的燃料生产设备,以藻类培养所需的水平输送二氧化碳。我们的研究表明,将 DAC 与该生物燃料生产设施集成,可带来成本和温室气体排放效益。热能集成可减少加热所需的能源需求,从而降低运营成本。大规模集成利用烟道气二氧化碳作为 PBR 的碳源,降低了 DAC 系统的规模,从而节省了资本和运营成本。最有利的方案取决于热量和质量集成的相互作用,同时还要使藻类生长的昼夜节律与 DAC 系统和燃料生产固有的稳定节奏和能源需求相匹配。就这些技术而言,DAC-PBR 质量和能量集成在当前技术水平下可降低 18% 的成本,减少 50% 的温室气体排放。
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来源期刊
Journal of CO2 Utilization
Journal of CO2 Utilization CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.90
自引率
10.40%
发文量
406
审稿时长
2.8 months
期刊介绍: The Journal of CO2 Utilization offers a single, multi-disciplinary, scholarly platform for the exchange of novel research in the field of CO2 re-use for scientists and engineers in chemicals, fuels and materials. The emphasis is on the dissemination of leading-edge research from basic science to the development of new processes, technologies and applications. The Journal of CO2 Utilization publishes original peer-reviewed research papers, reviews, and short communications, including experimental and theoretical work, and analytical models and simulations.
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