Graphene nanoplatelets on recycled rubber: an experimental study of material properties and mechanical improvements.

IF 4.3 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences Pub Date : 2024-10-23 Epub Date: 2024-09-09 DOI:10.1098/rsta.2023.0324
J M Londono Monsalve, E Kovalska, M F Craciun, M R Marsico
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Abstract

This study presents an experimental investigation of the mechanical behaviour of recycled rubber pads coated with graphene nanoplatelets. The investigation is part of an effort to develop a novel rubber-based composite that aims to reroute rubber from end-of-life tyres from illegal landfills and incineration back into the market in the form of a novel composite for vibration isolation. Graphene nanoplatelets were deposited on rubber pads via ultrasonic spray coating. The pads were made of a combination of recycled rubber (from tyres) and virgin rubber. A comprehensive analysis of the structural and chemical properties of the graphene coating, ensuring its integrity on the rubber substrate, was performed by combining surface topography, Raman and Fourier-transform infrared (FTIR) spectroscopy. Stacked coated pads were cured and tested dynamically in compression and shear under cyclic loading. Results showed promising improvements in the mechanical properties, in particular, in compressive stiffness and damping of the coated specimens with respect to their uncoated counterparts, laying the foundation for using graphene-enhanced recycled rubber as a novel composite.This article is part of the theme issue 'Celebrating the 15th anniversary of the Royal Society Newton International Fellowship'.

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再生橡胶上的石墨烯纳米颗粒:材料性能和机械改进的实验研究。
本研究对涂有石墨烯纳米颗粒的再生橡胶垫的机械性能进行了实验研究。这项研究是开发新型橡胶基复合材料工作的一部分,旨在将非法填埋和焚烧的报废轮胎中的橡胶以新型隔振复合材料的形式重新投入市场。石墨烯纳米颗粒通过超声波喷涂沉积在橡胶垫上。橡胶垫由再生橡胶(来自轮胎)和原生橡胶组合而成。通过结合表面形貌、拉曼和傅立叶变换红外(FTIR)光谱,对石墨烯涂层的结构和化学特性进行了全面分析,以确保其在橡胶基材上的完整性。堆叠涂层衬垫固化后,在循环加载下进行压缩和剪切动态测试。结果表明,与未涂覆的试样相比,涂覆试样的机械性能,特别是压缩刚度和阻尼有了很大改善,这为将石墨烯增强再生橡胶用作新型复合材料奠定了基础。
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来源期刊
CiteScore
9.30
自引率
2.00%
发文量
367
审稿时长
3 months
期刊介绍: Continuing its long history of influential scientific publishing, Philosophical Transactions A publishes high-quality theme issues on topics of current importance and general interest within the physical, mathematical and engineering sciences, guest-edited by leading authorities and comprising new research, reviews and opinions from prominent researchers.
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