Catalytic Heaters at Oil and Gas Sites May be a Significant yet Overlooked Seasonal Source of Methane Emissions

IF 8.9 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Environmental Science & Technology Letters Environ. Pub Date : 2024-08-12 DOI:10.1021/acs.estlett.4c0045310.1021/acs.estlett.4c00453
Simon A. Festa-Bianchet, Milad Mohammadikharkeshi, David R. Tyner and Matthew R. Johnson*, 
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Abstract

Successful reduction of oil and gas sector methane emissions to meet near-zero intensity targets requires the identification and mitigation of all possible sources. One potentially important source is catalytic heaters, which have largely escaped attention in regulatory and mitigation efforts despite being ubiquitous at upstream production sites in cold climate regions. This study reports direct in situ measurements of the exhaust streams of 38 natural gas-fired catalytic heaters at upstream production sites in British Columbia, Canada. All heaters in the sample showed consistently poor methane conversion with mean destruction efficiencies of 61 ± 5% while releasing 235 [+31/–28] g of methane per cubic meter of fuel. Although individual units are generally small methane sources (mean of 0.28 ± 0.04 kg/h), their prevalence means they could represent 6% of the total provincial upstream methane inventory and as an aggregate methane source could be 5× more significant than abandoned wells. Notably, these heaters are seasonal sources whose emissions would be missed in measurement campaigns occurring solely in summer months. However, additional measurements from a small number of heat medium burners demonstrate that, where feasible, methane emissions can be reduced by approximately 425× by replacing catalytic heaters with centralized heat systems.

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油气田催化加热器可能是一个重要但被忽视的季节性甲烷排放源
要成功减少石油和天然气行业的甲烷排放以实现近零强度目标,需要识别并减少所有可能的来源。催化加热器是一个潜在的重要来源,尽管它在寒冷气候地区的上游生产基地无处不在,但在监管和减排工作中却基本上没有受到关注。本研究报告对加拿大不列颠哥伦比亚省上游生产基地的 38 台天然气催化加热器的废气流进行了直接现场测量。样本中的所有加热器的甲烷转化率一直很低,平均破坏效率为 61 ± 5%,而每立方米燃料释放 235 [+31/-28] 克甲烷。虽然单个设备的甲烷来源一般较小(平均为 0.28 ± 0.04 千克/小时),但它们的普遍存在意味着它们可能占全省上游甲烷库存总量的 6%,作为一个甲烷总来源,其重要性可能是废弃水井的 5 倍。值得注意的是,这些加热器是季节性来源,仅在夏季进行的测量活动会漏掉它们的排放。然而,对少量热媒燃烧器的额外测量表明,在可行的情况下,用集中供热系统取代催化加热器可减少甲烷排放量约 425 倍。
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来源期刊
Environmental Science & Technology Letters Environ.
Environmental Science & Technology Letters Environ. ENGINEERING, ENVIRONMENTALENVIRONMENTAL SC-ENVIRONMENTAL SCIENCES
CiteScore
17.90
自引率
3.70%
发文量
163
期刊介绍: Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.
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