Broadband infrared imaging governed by guided-mode resonance in dielectric metasurfaces

IF 3.5 3区 医学 Q2 CHEMISTRY, MEDICINAL ACS Medicinal Chemistry Letters Pub Date : 2024-09-10 DOI:10.1038/s41377-024-01535-w
Ze Zheng, Daria Smirnova, Gabriel Sanderson, Ying Cuifeng, Demosthenes C. Koutsogeorgis, Lujun Huang, Zixi Liu, Rupert Oulton, Arman Yousefi, Andrey E. Miroshnichenko, Dragomir N. Neshev, Mary O’Neill, Mohsen Rahmani, Lei Xu
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Abstract

Nonlinear metasurfaces have experienced rapid growth recently due to their potential in various applications, including infrared imaging and spectroscopy. However, due to the low conversion efficiencies of metasurfaces, several strategies have been adopted to enhance their performances, including employing resonances at signal or nonlinear emission wavelengths. This strategy results in a narrow operational band of the nonlinear metasurfaces, which has bottlenecked many applications, including nonlinear holography, image encoding, and nonlinear metalenses. Here, we overcome this issue by introducing a new nonlinear imaging platform utilizing a pump beam to enhance signal conversion through four-wave mixing (FWM), whereby the metasurface is resonant at the pump wavelength rather than the signal or nonlinear emissions. As a result, we demonstrate broadband nonlinear imaging for arbitrary objects using metasurfaces. A silicon disk-on-slab metasurface is introduced with an excitable guided-mode resonance at the pump wavelength. This enabled direct conversion of a broad IR image ranging from >1000 to 4000 nm into visible. Importantly, adopting FWM substantially reduces the dependence on high-power signal inputs or resonant features at the signal beam of nonlinear imaging by utilizing the quadratic relationship between the pump beam intensity and the signal conversion efficiency. Our results, therefore, unlock the potential for broadband infrared imaging capabilities with metasurfaces, making a promising advancement for next-generation all-optical infrared imaging techniques with chip-scale photonic devices.

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介电元表面导模共振控制的宽带红外成像
非线性元表面因其在红外成像和光谱学等各种应用中的潜力,最近经历了快速发展。然而,由于元表面的转换效率较低,人们采用了多种策略来提高其性能,包括在信号波长或非线性发射波长上采用共振。这种策略导致非线性超表面的工作频带较窄,从而制约了许多应用,包括非线性全息、图像编码和非线性金属透镜。在这里,我们引入了一种新的非线性成像平台,利用泵浦光束通过四波混合(FWM)增强信号转换,从而使元表面在泵浦波长而非信号或非线性发射处产生共振,从而克服了这一问题。因此,我们利用元表面演示了任意物体的宽带非线性成像。我们在泵浦波长处引入了可激发导模共振的硅片盘元表面。这样就能将范围从 1000 纳米到 4000 纳米的宽红外图像直接转换为可见光图像。重要的是,通过利用泵浦光束强度与信号转换效率之间的二次关系,采用 FWM 技术大大降低了非线性成像对高功率信号输入或信号光束共振特征的依赖。因此,我们的研究结果释放了利用超表面实现宽带红外成像功能的潜力,为利用芯片级光子器件实现下一代全光红外成像技术带来了希望。
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来源期刊
ACS Medicinal Chemistry Letters
ACS Medicinal Chemistry Letters CHEMISTRY, MEDICINAL-
CiteScore
7.30
自引率
2.40%
发文量
328
审稿时长
1 months
期刊介绍: ACS Medicinal Chemistry Letters is interested in receiving manuscripts that discuss various aspects of medicinal chemistry. The journal will publish studies that pertain to a broad range of subject matter, including compound design and optimization, biological evaluation, drug delivery, imaging agents, and pharmacology of both small and large bioactive molecules. Specific areas include but are not limited to: Identification, synthesis, and optimization of lead biologically active molecules and drugs (small molecules and biologics) Biological characterization of new molecular entities in the context of drug discovery Computational, cheminformatics, and structural studies for the identification or SAR analysis of bioactive molecules, ligands and their targets, etc. Novel and improved methodologies, including radiation biochemistry, with broad application to medicinal chemistry Discovery technologies for biologically active molecules from both synthetic and natural (plant and other) sources Pharmacokinetic/pharmacodynamic studies that address mechanisms underlying drug disposition and response Pharmacogenetic and pharmacogenomic studies used to enhance drug design and the translation of medicinal chemistry into the clinic Mechanistic drug metabolism and regulation of metabolic enzyme gene expression Chemistry patents relevant to the medicinal chemistry field.
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