Impact of biological environment on bending fatigue lifetime in additive-manufactured polylactic acid fabricated by 3D-printing

IF 5 2区 材料科学 Q1 MATERIALS SCIENCE, CHARACTERIZATION & TESTING Polymer Testing Pub Date : 2024-09-01 DOI:10.1016/j.polymertesting.2024.108562
Fatemeh Zahra Hosseini, Morteza Kianifar, Mohammad Azadi
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Abstract

Polylactic acid (PLA) has become desirable for biomedical applications, particularly implantable devices. However, the degradation of PLA in biological environments under mechanical stress remains incompletely understood and requires further investigation. This study compared the plain fatigue (PF) and the biodegraded fatigue (BDF) behavior of 3D-printed PLA. For this purpose, two sets of standard fatigue specimens were additively manufactured by the fused filament fabrication (FFF) method. One set was used for plain fatigue testing, and the other was immersed for 330 days in simulated body fluid (SBF). After immersion, the samples were dried and weighed before fatigue testing. The fully reversed rotary bending fatigue tests were conducted on both sets of specimens, and the stress-lifetime (S-N) curves were obtained. Additionally, the fatigue properties of PF and BDF specimens were evaluated. Moreover, the fracture behaviors of the materials were studied using field emission scanning electron microscopy (FESEM). The outcomes implied that the weight of the samples extended during the immersion period, primarily due to water absorption by the PLA. However, after drying, the final weights did not change compared to the weights before immersion. The SBF immersion significantly reduced the fatigue performance of the biodegraded samples comparing the PF result.

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生物环境对三维打印增材制造聚乳酸弯曲疲劳寿命的影响
聚乳酸(PLA)已成为生物医学应用的理想材料,尤其是植入式设备。然而,人们对聚乳酸在生物环境中机械应力作用下的降解情况仍不甚了解,需要进一步研究。本研究比较了三维打印聚乳酸的普通疲劳(PF)和生物降解疲劳(BDF)行为。为此,采用熔融长丝制造(FFF)方法添加制造了两组标准疲劳试样。一组用于普通疲劳测试,另一组在模拟体液(SBF)中浸泡 330 天。浸泡后,样品在疲劳测试前进行干燥和称重。两组试样都进行了完全反转的旋转弯曲疲劳试验,并得到了应力-寿命(S-N)曲线。此外,还评估了 PF 和 BDF 试样的疲劳特性。此外,还使用场发射扫描电子显微镜(FESEM)研究了材料的断裂行为。结果表明,样品的重量在浸泡期间有所增加,这主要是由于聚乳酸的吸水性。然而,干燥后的最终重量与浸泡前的重量相比没有变化。与 PF 结果相比,SBF 浸泡大大降低了生物降解样品的疲劳性能。
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来源期刊
Polymer Testing
Polymer Testing 工程技术-材料科学:表征与测试
CiteScore
10.70
自引率
5.90%
发文量
328
审稿时长
44 days
期刊介绍: Polymer Testing focuses on the testing, analysis and characterization of polymer materials, including both synthetic and natural or biobased polymers. Novel testing methods and the testing of novel polymeric materials in bulk, solution and dispersion is covered. In addition, we welcome the submission of the testing of polymeric materials for a wide range of applications and industrial products as well as nanoscale characterization. The scope includes but is not limited to the following main topics: Novel testing methods and Chemical analysis • mechanical, thermal, electrical, chemical, imaging, spectroscopy, scattering and rheology Physical properties and behaviour of novel polymer systems • nanoscale properties, morphology, transport properties Degradation and recycling of polymeric materials when combined with novel testing or characterization methods • degradation, biodegradation, ageing and fire retardancy Modelling and Simulation work will be only considered when it is linked to new or previously published experimental results.
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