Correlating scatterer concentration and intensity threshold of random laser in niobium oxide particle colloids with dye solution

IF 3.8 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Optical Materials Pub Date : 2024-09-05 DOI:10.1016/j.optmat.2024.116072
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Abstract

Our study examines how the concentration of scatterers affects the intensity threshold of random laser (RL) action in colloids made of niobium oxide particles and Rhodamine B dye. This is the first reported instance of RL action in niobium oxide. We kept the dye (gain medium) concentration constant and quantified how varying concentrations of niobium oxide particles (scatterers) affect the RL intensity threshold. Our findings indicate an inverse relationship between the concentration of niobium oxide particles and the RL threshold. Increasing the niobium oxide concentration from 0.32 mM to 2.50 mM decreased the RL threshold by up to 70 %, suggesting that higher scatterer densities lead to enhanced efficiency of the lasing process. We noticed that the RL intensity thresholds decrease concerning scatterer concentration, highlighting the significant impact of scatterer density on lasing efficiency. These results could provide a better comprehension of the mechanics of RL in disordered media and emphasize the essential role of scatterer density in determining RL efficiency. Our work deepens the understanding of RL dynamics and lays the groundwork for designing and optimizing colloidal RL systems for various applications such as imaging and optical sensing.

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氧化铌颗粒胶体中散射体浓度与随机激光强度阈值与染料溶液的相关性
我们的研究探讨了散射体的浓度如何影响由氧化铌颗粒和罗丹明 B 染料组成的胶体中随机激光(RL)作用的强度阈值。这是首次报道氧化铌中的随机激光作用。我们保持染料(增益介质)浓度不变,并量化了不同浓度的氧化铌颗粒(散射体)如何影响 RL 强度阈值。我们的研究结果表明,氧化铌颗粒的浓度与 RL 阈值之间存在反比关系。将氧化铌的浓度从 0.32 mM 提高到 2.50 mM,可使 RL 门限降低 70%,这表明较高的散射体密度可提高激光过程的效率。我们注意到,RL 强度阈值随着散射体浓度的增加而降低,这凸显了散射体密度对激光效率的重要影响。这些结果有助于更好地理解无序介质中的 RL 力学,并强调了散射体密度在决定 RL 效率方面的重要作用。我们的工作加深了对 RL 动态的理解,为设计和优化胶体 RL 系统以用于成像和光学传感等各种应用奠定了基础。
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来源期刊
Optical Materials
Optical Materials 工程技术-材料科学:综合
CiteScore
6.60
自引率
12.80%
发文量
1265
审稿时长
38 days
期刊介绍: Optical Materials has an open access mirror journal Optical Materials: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. The purpose of Optical Materials is to provide a means of communication and technology transfer between researchers who are interested in materials for potential device applications. The journal publishes original papers and review articles on the design, synthesis, characterisation and applications of optical materials. OPTICAL MATERIALS focuses on: • Optical Properties of Material Systems; • The Materials Aspects of Optical Phenomena; • The Materials Aspects of Devices and Applications. Authors can submit separate research elements describing their data to Data in Brief and methods to Methods X.
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