Thermal and mechanical behaviour of recycled short milled carbon fibre reinforced polypropylene and recycled polypropylene composites: A comparative study

Yitao Zheng, Fu Gu, Bin Wang, Zheng Wang, Chuang Gao, Yun Zhou, Philip Hall
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Abstract

Environmental and economic factors have driven research into the recycling and applications of recycled carbon fibres (rCF). This paper presents a comparative study characterizing and comparing the mechanical and thermal performance of recycled short milled carbon fibre (rSMCF) on virgin and recycled polypropylene composites. The effects of rSMCF on VPP and RPP on mechanical performance were analysed and compared. At 5 wt% rSMCF, recycled polypropylene achieved 52.3% and 47.3% improvement on tensile and flexural modulus, while at the same rSMCF loading, virgin polypropylene only improved 37.7% and 17.5%, respectively. The un-notched impact strength of RPP-based composites reduced from 83.2 kJ/m to 60.1 kJ/m when rSMCF content increased from 1 wt% to 5 wt%, indicating future work should enhance the fibre/polymer interface performance. Crystal contents () of the PP/rSMCF composites were investigated by differential scanning calorimetry (DSC), and the results were analysed and mapped to the mechanical performance. The results of this study propose a novel scalable method for the production of high-performance VPP/RPP composite materials using rSMCF.
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再生短磨碳纤维增强聚丙烯和再生聚丙烯复合材料的热性能和机械性能:比较研究
环境和经济因素推动了对回收碳纤维(rCF)的回收和应用的研究。本文介绍了一项比较研究,对再生短磨碳纤维(rSMCF)在原生和再生聚丙烯复合材料上的机械性能和热性能进行了表征和比较。研究分析并比较了 rSMCF 对 VPP 和 RPP 对机械性能的影响。在 5 wt% 的 rSMCF 下,再生聚丙烯的拉伸和弯曲模量分别提高了 52.3% 和 47.3%,而在相同的 rSMCF 负载下,原生聚丙烯仅分别提高了 37.7% 和 17.5%。当 rSMCF 含量从 1 wt% 增加到 5 wt% 时,基于 RPP 的复合材料的无缺口冲击强度从 83.2 kJ/m 降至 60.1 kJ/m,这表明未来的工作应提高纤维/聚合物界面的性能。通过差示扫描量热法(DSC)研究了 PP/rSMCF 复合材料的晶体含量(),并分析了结果与机械性能的关系。研究结果提出了一种利用 rSMCF 生产高性能 VPP/RPP 复合材料的新型可扩展方法。
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