Detailed numerical simulation and experiments of a steadily burning micron-sized aluminum droplet in hot steam-dominated flows

IF 5.3 2区 工程技术 Q2 ENERGY & FUELS Proceedings of the Combustion Institute Pub Date : 2024-08-22 DOI:10.1016/j.proci.2024.105717
Yue Qiu, Sheng Feng, Zhiyong Wu, Shijie Xu, Can Ruan, Xue-Song Bai, Elna J.K. Nilsson, Marcus Aldén, Zhongshan Li
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Abstract

Detailed numerical simulations are conducted in comparison with experimental results to study the flame structure and burning rate of a steadily burning aluminum droplet in hot steam-dominated environments. The droplet surface temperature, flame temperature, and flame stabilization position are measured along with the droplet burning rate estimated from the droplet size evolution. A numerical model accounting for detailed transport properties and chemical kinetics is presented and applied to unveil the flame structure, species and temperature distributions, and heat/mass transfer between the droplet and the surrounding gas. The numerical results of the temperature, velocity, and species distribution profiles demonstrate that the aluminum vapor flame is of classical diffusion flame structure, where near the droplet, there is a non-negligible amount of AlOAl apart from the main product AlO. This supports the deposition and formation of an alumina cap on the surface proposed in the literature. The simulation correctly captured the flame temperature and flame stabilization distance for a range of droplet sizes. Net heat flux analysis shows that conduction heat from the flame front accounts for less than 30% of the heat needed in aluminum evaporation, which warrants further quantification on other heat sources. The experimental and numerical results enrich the knowledge of the heat/mass transfer and chemical reactions near the droplet, which helps deepen the understanding of aluminum droplet burning.
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热蒸汽主导流中稳定燃烧的微米级铝液滴的详细数值模拟和实验
通过详细的数值模拟与实验结果对比,研究了在热蒸汽为主的环境中稳定燃烧的铝液滴的火焰结构和燃烧速率。在测量液滴表面温度、火焰温度和火焰稳定位置的同时,还测量了根据液滴大小变化估算出的液滴燃烧速率。介绍并应用了一个考虑到详细传输特性和化学动力学的数值模型,以揭示火焰结构、物种和温度分布以及液滴与周围气体之间的热量/质量传递。温度、速度和物种分布曲线的数值结果表明,铝蒸气火焰是典型的扩散火焰结构,在液滴附近,除了主要产物 AlO 外,还有不可忽略的 AlOAl。这支持了文献中提出的在表面沉积并形成氧化铝帽的观点。模拟正确捕捉到了一系列液滴大小的火焰温度和火焰稳定距离。净热流量分析表明,来自火焰前沿的传导热量只占铝蒸发所需热量的不到 30%,因此需要进一步量化其他热源。实验和数值结果丰富了对液滴附近热量/质量传递和化学反应的认识,有助于加深对铝液滴燃烧的理解。
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来源期刊
Proceedings of the Combustion Institute
Proceedings of the Combustion Institute 工程技术-工程:化工
CiteScore
7.00
自引率
0.00%
发文量
420
审稿时长
3.0 months
期刊介绍: The Proceedings of the Combustion Institute contains forefront contributions in fundamentals and applications of combustion science. For more than 50 years, the Combustion Institute has served as the peak international society for dissemination of scientific and technical research in the combustion field. In addition to author submissions, the Proceedings of the Combustion Institute includes the Institute''s prestigious invited strategic and topical reviews that represent indispensable resources for emergent research in the field. All papers are subjected to rigorous peer review. Research papers and invited topical reviews; Reaction Kinetics; Soot, PAH, and other large molecules; Diagnostics; Laminar Flames; Turbulent Flames; Heterogeneous Combustion; Spray and Droplet Combustion; Detonations, Explosions & Supersonic Combustion; Fire Research; Stationary Combustion Systems; IC Engine and Gas Turbine Combustion; New Technology Concepts The electronic version of Proceedings of the Combustion Institute contains supplemental material such as reaction mechanisms, illustrating movies, and other data.
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