Porphyrin-linked graphdiyne as a substrate for constructing single-atom catalysts with transition metals towards oxygen reduction reactions and oxygen evolution reactions†

IF 6 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Materials Chemistry Frontiers Pub Date : 2024-08-31 DOI:10.1039/D4QM00555D
Jiejie Ping, Mei Wu, Manyu Liu, Yan Jiang, Wenhui Shang, Menggai Jiao, Jiahao Ruan, Nan Wang and Zhiyu Jia
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Abstract

Porphyrin-linked graphdiyne (PGDY) is a carbon-based material that provides a platform for anchoring single-atom catalysts (SACs) with transition metals (TMs). These SACs have the potential to boost the catalytic activity of the PGDY substrate. The synthesized TM@PGDY composites showed remarkable catalytic activity towards oxygen reduction reactions and oxygen evolution reactions.

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以连接卟啉的石墨二炔为底物,用过渡金属构建单原子催化剂,用于氧还原反应和氧进化反应
卟啉连接的石墨二乙烯(PGDY)是一种碳基材料,为过渡金属(TM)锚定单原子催化剂(SAC)提供了平台。这些单原子催化剂具有提高 PGDY 底物催化活性的潜力。合成的 TM@PGDY 复合材料在氧还原反应和氧进化反应中表现出显著的催化活性。
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来源期刊
Materials Chemistry Frontiers
Materials Chemistry Frontiers Materials Science-Materials Chemistry
CiteScore
12.00
自引率
2.90%
发文量
313
期刊介绍: Materials Chemistry Frontiers focuses on the synthesis and chemistry of exciting new materials, and the development of improved fabrication techniques. Characterisation and fundamental studies that are of broad appeal are also welcome. This is the ideal home for studies of a significant nature that further the development of organic, inorganic, composite and nano-materials.
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