Moiré Kramers-Weyl Fermions from Structural Chirality with Ideal Radial Spin Texture

Abstract

We demonstrate that two-dimensional Kramers-Weyl fermions can be engineered in spin-orbit coupled twisted bilayers, where the chiral structure of these moir\'e systems breaks all mirror symmetries, confining Kramers-Weyl fermions to high-symmetry points in the Brillouin zone under time reversal symmetry. Our theoretical analysis reveals a symmetry-enforced Weyl-like interlayer moir\'e coupling that universally ensures an ideal radial spin-texture at arbitrary twist angles, under $C_{nz}$ symmetry with n>2. First principles density functional calculation confirm the realization of these fermions in twisted $\alpha$-In$_2$Se$_3$ bilayers, where flat bands and out-of-plane ferroelectric polarization in each layer guarantee two-dimensional Kramers-Weyl physics with perfectly ideal radial spin textures.