The nature of water interactions and the molecular signatures of hydrophilicity

Nicolás A. Loubet, Alejandro R. Verde, Gustavo A. Appignanesi
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Abstract

The peculiar structuring of liquid water stems from a fine-tuned molecular principle embodying the two different interaction demands of the water molecule: The formation of hydrogen bonds or the compensation for coordination defects. Here we shall show that the same underlying molecular mechanism is also at play in order to establish favorable interactions with other systems. In this regard, the emergence of two limiting behaviors for hydrophilicity will help both to unravel its molecular underpinnings and to establish absolute values for such property.
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水相互作用的性质和亲水性的分子特征
液态水的奇特结构源于一个微调的分子原理,它体现了水分子两种不同的相互作用需求:氢键的形成或配位缺陷的补偿。在这里,我们将证明,为了与其他体系建立有利的相互作用,同样的潜在分子机制也在起作用。在这方面,亲水性的两种极限行为的出现将有助于揭示其分子基础,并为这种性质确定绝对值。
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