Spontaneous imbibition in hydrate-bearing sediments under creep

0 ENERGY & FUELS Gas Science and Engineering Pub Date : 2024-09-16 DOI:10.1016/j.jgsce.2024.205452
Kailun Wang , Gang Lei , Jiangtao Qu , Yang Wu , Wan Cheng , Jiadi Tang , Yuyi Lu
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Abstract

During hydrate exploitation, water generated by the phase transition of natural gas hydrate (NGH) invades the pore space of hydrate-bearing sediments (HBS) through spontaneous imbibition (SI), restricting the depressurization-based extraction. Besides, the creep behaviors of HBS complicate the SI process. Therefore, it is crucial to understand SI behaviors in HBS under creep. This study presents a theoretical model considering the effects of creep behaviors of HBS due to effective stress, as well as occurrence patterns and saturation of NGH. Moreover, fracture networks generation due to hydration in HBS, wall roughness, gravity, and dynamic contact angle are considered. The proposed model is adequately validated by available experimental data. In addition, based on the derived model, parameter sensitivity analysis is carried out. The results demonstrate that the porosity and wall roughness of HBS significantly enhance the SI capacity of HBS. Moreover, when other parameters are fixed, the SI capacity decreases with the increase of hydrate saturation (or retained water saturation). In addition, during the creep process, the SI capacity decreases with time. The derived model not only helps to better understand and predict the SI kinetics in gas hydrate reservoirs, but also provides guidance for the hydrate exploitation process.

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蠕变条件下含水沉积物的自发浸润
在水合物开采过程中,天然气水合物(NGH)相变产生的水通过自发浸润(SI)侵入含水沉积物(HBS)的孔隙空间,限制了基于减压的开采。此外,含水层沉积物的蠕变行为也使 SI 过程变得复杂。因此,了解蠕变条件下 HBS 的 SI 行为至关重要。本研究提出了一个理论模型,考虑了有效应力对 HBS 蠕变行为的影响,以及 NGH 的发生模式和饱和度。此外,还考虑了因 HBS 中的水化作用、壁面粗糙度、重力和动态接触角而产生的断裂网络。现有的实验数据充分验证了所提出的模型。此外,基于推导出的模型,还进行了参数敏感性分析。结果表明,HBS 的孔隙率和壁面粗糙度能显著提高 HBS 的 SI 能力。此外,当其他参数固定时,SI 容量会随着水合物饱和度(或保留水饱和度)的增加而降低。此外,在蠕变过程中,SI 容量会随着时间的推移而降低。推导出的模型不仅有助于更好地理解和预测天然气水合物储层的 SI 动力学,还能为水合物开采过程提供指导。
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