Origin of the non-Fermi-liquid behavior in CeRh2As2

P. Khanenko, D. Hafner, K. Semeniuk, J. Banda, T. Luehmann, F. Baertl, T. Kotte, J. Wosnitza, G. Zwicknagl, C. Geibel, J. F. Landaeta, S. Khim, E. Hassinger, M. Brando
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Abstract

Unconventional superconductivity in heavy-fermion systems appears often near magnetic quantum critical points (QCPs). This seems to be the case also for CeRh2As2 (Tc $\approx$ 0.31 K). CeRh2As2 shows two superconducting (SC) phases, SC1 and SC2, for a magnetic field along the c axis of the tetragonal unit cell, but only the SC1 phase is observed for a field along the basal plane. Furthermore, another ordered state (phase-I) is observed below T0 $\approx$ 0.48 K whose nature is still unclear: Thermodynamic and magnetic measurements pointed to a non magnetic multipolar state, but recent $\mu$SR and NQR/NMR experiments have clearly detected antiferromagnetic (AFM) order below T0 . Also, quasi-two-dimensional AFM fluctuations were observed in NMR and neutron-scattering experiments above T0. The proximity of a QCP is indicated by non-Fermi-liquid (NFL) behavior observed above the ordered states in both specific heat $C(T)/T \propto T^{-0.6}$ and resistivity $\rho(T) \propto T^{0.5}$. These T-dependencies are not compatible with any generic AFM QCP. Because of the strong magnetic-field anisotropy of both the SC phase and phase I, it is possible to study a field-induced SC QCP as well a phase-I QCP by varying the angle $\alpha$ between the field and the c axis. Thus, by examining the behavior of the electronic specific-heat coefficient C(T)/T across these QCPs, we can determine which phase is associated with the NFL behavior. Here, we present low-temperature specific-heat measurements taken in a magnetic field as high as 21 T applied at several angles $\alpha$. We observe that the NFL behavior does very weakly depend on the field and on the angle $\alpha$, a result that is at odd with that observations in standard magnetic QCPs. This suggests a nonmagnetic origin of the quantum critical fluctuations.
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CeRh2As2 中非费米液体行为的起源
重费米子系统中的非常规超导性通常出现在磁性量子临界点(QCPs)附近。CeRh2As2 似乎也是这种情况(Tc $\approx$ 0.31 K)。CeRh2As2显示出两种超导(SC)相:SC1和SC2,磁场沿四方晶胞的c轴方向,但只有SC1相在磁场沿基底面方向时被观察到。此外,在 T0 $\approx$0 以下还观察到另一种有序态(phase-I),其性质尚不清楚:热力学和磁学测量结果表明这是一种非磁性多极态,但最近的 $\mu$SR 和 NQR/NMR 实验清楚地检测到了 T0 以下的反铁磁(AFM)有序态。在有序态之上观察到的非费米液体(NFL)行为表明,在有序态之上的比热 $C(T)/T \propto T^{-0.6}$ 和电阻率 $\rho(T) \proptoT^{0.5}$ 都接近 QCP。由于 SC 相和 I 相都具有很强的磁场各向异性,因此可以通过改变磁场与 c 轴之间的角度 $\alpha$ 来研究磁场诱导的 SC QCP 以及 I 相 QCP。因此,通过研究电子比热系数 C(T)/T 在这些 QCP 上的行为,我们可以确定哪一相与 NFL 行为相关。在这里,我们展示了在 21 T 的高磁场中以多个角度 $\alpha$ 进行的低温比热测量。我们观察到,NFL 行为确实非常微弱地依赖于磁场和角度 $\alpha$,这一结果与在标准磁性 QCP 中观察到的结果截然不同。这表明量子临界波动起源于非磁性。
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