Local-field corrections of the Green's tensor in chiral media

IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Physical Review A Pub Date : 2024-09-16 DOI:10.1103/physreva.110.033109
Janine C. Franz, Stefan Yoshi Buhmann, A. Salam
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Abstract

In this paper we derive local-field corrections for interactions within chiral media using the Onsager real cavity model. The problem is not fully solvable analytically, so we introduce a matrix formalism to determine the correct local-field corrections. We find that left- and right-handed circularly polarized excitations yield different correction factors inside a chiral medium, analogous to their different propagation velocities. These chiral correction factors can significantly alter theoretical predictions for chiral effects within the medium. We validate our solution in various limits and special cases, particularly when the source and absorption points coincide, enabling analytical comparison for nonabsorbing media. For spontaneous emission in a chiral medium, we extend the local-field correction to absorbing media, revealing fundamentally different corrections analogous to the nonchiral case.

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手性介质中格林张量的局部场修正
在本文中,我们利用昂萨格实腔模型推导了手性介质内相互作用的局域场修正。这个问题无法完全通过解析求解,因此我们引入矩阵形式来确定正确的局域场修正。我们发现,左旋和右旋圆极化激波在手性介质中会产生不同的修正系数,类似于它们不同的传播速度。这些手性修正因子会显著改变介质内部手性效应的理论预测。我们在各种限制和特殊情况下验证了我们的解决方案,特别是当源点和吸收点重合时,可以对非吸收介质进行分析比较。对于手性介质中的自发辐射,我们将局域场修正扩展到吸收介质,揭示了与非手性情况类似的根本不同的修正。
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来源期刊
Physical Review A
Physical Review A 物理-光学
CiteScore
5.40
自引率
24.10%
发文量
0
审稿时长
2.2 months
期刊介绍: Physical Review A (PRA) publishes important developments in the rapidly evolving areas of atomic, molecular, and optical (AMO) physics, quantum information, and related fundamental concepts. PRA covers atomic, molecular, and optical physics, foundations of quantum mechanics, and quantum information, including: -Fundamental concepts -Quantum information -Atomic and molecular structure and dynamics; high-precision measurement -Atomic and molecular collisions and interactions -Atomic and molecular processes in external fields, including interactions with strong fields and short pulses -Matter waves and collective properties of cold atoms and molecules -Quantum optics, physics of lasers, nonlinear optics, and classical optics
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