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Combined microwave and optical spectroscopy for hyperfine structure analysis in thulium atoms 结合微波和光学光谱分析铥原子的超精细结构
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-19 DOI: 10.1103/physreva.110.032817
Denis Mishin, Dmitry Tregubov, Nikolay Kolachevsky, Artem Golovizin
We present refined values of the hyperfine splitting frequencies of the ground |g=|4f13(2Fo)6s2,J=7/2 and clock |c=|4f13(2Fo)6s2,J=5/2 states of thulium atoms, fgHFS=1496550658.23(3) Hz and fcHFS=2113946873.08(9) Hz, respectively. The measurements are performed on an ultracold atomic ensemble in an optical lattice using combined microwave and optical transition spectroscopy. The achieved measurement accuracy of less than 0.1 ppb represents an improvement of 2 and 7 orders of magnitude for fgHFS and fcHFS, respectively, compared to the previously published values. We also refine the value of the Landé g-factor of the clock level to gc=0.854786(12). The results of this work can be used in the frequency standards and quantum simulators based on thulium atoms being developed today, as well as in a number of fundamental studies that require precise knowledge of the hyperfine structure characteristics of various elements.
我们给出了铥原子基态|g〉=|4f13(2Fo)6s2,J=7/2〉和钟态|c〉=|4f13(2Fo)6s2,J=5/2〉的超细分裂频率的改进值,分别为fgHFS=1496550658.23(3) Hz和fcHFS=2113946873.08(9) Hz。测量是在光学晶格中的超冷原子集合上进行的,使用的是微波和光学跃迁光谱联合技术。与之前公布的数值相比,fgHFS 和 fcHFS 的测量精度小于 0.1 ppb,分别提高了 2 个和 7 个数量级。我们还将时钟电平的兰德 g 因子值改进为 gc=0.854786(12)。这项工作的结果可用于目前正在开发的基于铥原子的频率标准和量子模拟器,以及一些需要精确了解各种元素超正弦结构特征的基础研究。
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引用次数: 0
Spectral evidence of vibronic Rabi oscillations in the resonance-enhanced photodissociation of MgH+ 共振增强型光解离 MgH+ 中振动拉比振荡的光谱证据
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-19 DOI: 10.1103/physreva.110.033112
Dilfuza Umarova, Otabek Umarov, Attila Tóth, András Csehi
We study by real-time wave-packet simulations the sequential two-photon dissociation of the MgH+ molecule, under intense ultraviolet laser pulses of narrow spectral width. By a resonant coupling, one-photon Rabi oscillations are generated between two vibrational levels of the molecule, belonging to two different bound electronic states. These vibronic Rabi oscillations are probed upon absorption of further photons from the same laser pulse, that gradually promote the molecule to a dissociative electronic state. Calculating the energy spectrum of the photofragments explicitly analytically, we elucidate the physical origin of the main spectral features—such as the splitting, shifting, asymmetry, and multipeak pattern—identified by accurate numerical simulations. We find that the pronounced spectral intensity modulations result from the interference of fragment amplitudes that are generated during the distinct Rabi cycles in the upper and lower dynamically dressed states, formed upon the resonant coupling with the laser pulse. These intensity modulations are sensitively influenced by the resonant and nonresonant Stark effects, and can be manipulated by the parameters of the applied laser pulse. Our results contribute to the understanding and control of ultrafast coherent phenomena via the energy spectrum of particles emitted during the dynamical process under investigation.
我们通过实时波包模拟研究了 MgH+ 分子在窄光谱宽度的强紫外激光脉冲下的顺序双光子解离。通过共振耦合,分子的两个振动级(属于两个不同的束缚电子态)之间产生了单光子拉比振荡。在吸收来自同一激光脉冲的更多光子后,这些振动拉比振荡会被探测到,这些光子会逐渐促进分子进入解离电子态。通过明确分析计算光子碎片的能谱,我们阐明了主要光谱特征的物理来源--如分裂、移动、不对称和多峰模式--这些特征是通过精确的数值模拟确定的。我们发现,明显的光谱强度调制产生于碎片振幅的干扰,而碎片振幅是在与激光脉冲共振耦合后形成的上层和下层动态敷料态的不同拉比周期中产生的。这些强度调制会受到共振和非共振斯塔克效应的敏感影响,并可通过应用激光脉冲的参数进行操控。我们的研究结果有助于通过研究动态过程中发射的粒子能谱来理解和控制超快相干现象。
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引用次数: 0
Relativistic and recoil corrections to vacuum polarization in muonic systems: Three-photon exchange, gauge invariance, and numerical values μ介子系统真空极化的相对论修正和反冲修正:三光子交换、规规不变性和数值
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-19 DOI: 10.1103/physreva.110.032816
Gregory S. Adkins, Ulrich D. Jentschura
For an accurate theoretical description of muonic bound systems, it is crucial to consistently treat relativistic and recoil corrections to vacuum polarization. The one-loop vacuum-polarization effect is by far the dominant quantum electrodynamic (QED) energy correction for bound muons, being of order α(Zα)2mr, where α is the fine-structure constant, Z is the nuclear charge number, and mr is the reduced mass. Gauge invariance of the relativistic and recoil corrections to vacuum polarization of order α(Zα)4mr is investigated with respect to nonretarded and standard, renormalized variants of Coulomb gauge. The invariance is shown after including three-photon exchange diagrams. Our derivation is based on an adapted form of nonrelativistic quantum electrodynamics for bound muon systems (NRQEDμ), which is a version of NRQED where the hard scale is set at the muon mass instead of the electron mass. Updated values for the gauge-independent corrections for one-muon ions with nuclear charge numbers Z=1,2,6 are presented.
要对μ介子束缚系统进行准确的理论描述,关键是要始终如一地处理真空极化的相对论修正和反冲修正。一环真空极化效应是迄今为止束缚μ介子最主要的量子电动力学(QED)能量修正,其数量级为α(Zα)2mr,其中α是精细结构常数,Z是核电荷数,mr是还原质量。研究了阶数为α(Zα)4mr 的真空极化的相对论修正和反冲修正在库仑计的非保留和标准重规范化变体方面的量纲不变性。在包括三光子交换图之后,我们发现了其不变性。我们的推导基于针对束缚μ介子系统的非相对论量子电动力学(NRQEDμ)的改编形式,这是 NRQED 的一个版本,其中硬尺度设置为μ介子质量而不是电子质量。本文给出了核电荷数为 Z=1,2,6 的一介子离子的量规无关修正的最新值。
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引用次数: 0
Universality and two-body losses: Lessons from the effective non-Hermitian dynamics of two particles 普遍性和两体损失:从两个粒子的有效非赫米提动力学中汲取的教训
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-19 DOI: 10.1103/physreva.110.033321
Alice Marché, Hironobu Yoshida, Alberto Nardin, Hosho Katsura, Leonardo Mazza
We study the late-time dynamics of two particles confined in one spatial dimension and subject to two-body losses. The dynamics is exactly described by a non-Hermitian Hamiltonian that can be analytically studied both in the continuum and on a lattice. The asymptotic decay rate and the universal power-law form of the decay of the number of particles are exactly computed in the whole parameter space of the problem. When in the initial state the two particles are far apart, the average number of particles in the setup decays with time t as t1/2; a different power law, t3/2, is found when the two particles overlap in the initial state. These results are valid both in the continuum and on a lattice, but in the latter case a logarithmic correction appears.
我们研究了限制在一个空间维度并受到双体损耗的两个粒子的晚期动力学。该动力学由非赫米特哈密顿精确描述,可在连续体和晶格上进行分析研究。在问题的整个参数空间中,粒子数量的渐进衰减率和衰减的普遍幂律形式都是精确计算出来的。当初始状态中的两个粒子相距甚远时,设置中粒子的平均数量随时间 t 的衰减为 t-1/2;当初始状态中的两个粒子重叠时,发现了不同的幂律,即 t-3/2。这些结果在连续体和晶格上都有效,但在后一种情况下会出现对数修正。
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引用次数: 0
Multipartite multiplexing strategies for quantum routers 量子路由器的多方复用策略
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-18 DOI: 10.1103/physreva.110.032617
Julia A. Kunzelmann, Hermann Kampermann, Dagmar Bruß
This work explores the important role of quantum routers in communication networks and investigates the increase in efficiency using memories and multiplexing strategies. Motivated by the bipartite setup introduced by Abruzzo et al. [Phys. Rev. A 89, 012303 (2014)] for finite-range multiplexing in quantum repeaters, we extend the study to an N-partite network with a router as a central station. We present a general protocol for N parties after defining the underlying matching problem and we calculate the router rate for different N. We analyze the improvement due to multiplexing and analyze the secret key rate with explicit results for the tripartite network. Investigating strategic qubit selection for the Greenberger-Horne-Zeilinger measurements, we show that using cutoffs to remove qubits after a certain number of rounds and consistently combining qubits with the lowest number of storage rounds leads to an optimal secret key rate.
这项研究探讨了量子路由器在通信网络中的重要作用,并研究了利用存储器和复用策略提高效率的问题。受 Abruzzo 等人[Phys. Rev. A 89, 012303 (2014)]介绍的量子中继器中有限范围复用的两方设置的启发,我们将研究扩展到以路由器为中心站的 N 方网络。在定义了底层匹配问题之后,我们提出了一个适用于 N 方的通用协议,并计算了不同 N 的路由器速率。我们分析了多路复用带来的改进,并用三方网络的明确结果分析了秘钥速率。在研究格林伯格-霍恩-蔡林格测量的策略性量子比特选择时,我们表明,在一定轮数后使用截止来移除量子比特,并持续组合存储轮数最少的量子比特,可以获得最佳秘钥率。
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引用次数: 0
Parallel two-qubit entangling gates via a quantum nondemolition interaction controlled by rotation 通过旋转控制的量子非爆破相互作用实现并行双量子比特纠缠门
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-18 DOI: 10.1103/physreva.110.032616
E. A. Vashukevich, T. Yu. Golubeva
The paper presents an analysis of entangling and nonlocal operations in a quantum nondemolition (QND) interaction between multimode light with orbital angular momentum and an atomic ensemble. A protocol consists of two QND operations with rotations of quadratures of atomic spin coherence and light between them. This protocol provides a wide range of two-qubit operations, while the multimode nature of the chosen degrees of freedom allows the implementation of parallel operations over multiple two-qubit systems. We have used the formalism of equivalence classes and local invariants to evaluate the properties of two-qubit transformations. It is shown that, when selecting suitable values of the governing parameters, such as the duration of each of the two QND interactions and the rotation angles of the qubits, the protocol allows to realize a deterministic nonlocal SWAP operation and entangling SWAP operation with probability 13.
本文分析了具有轨道角动量的多模光与原子集合之间的量子非爆破(QND)相互作用中的纠缠和非局部操作。一个协议由两个 QND 操作组成,原子自旋相干性和光的四次方在它们之间旋转。该协议提供了广泛的双量子比特操作,而所选自由度的多模性质允许在多个双量子比特系统上实施并行操作。我们使用等价类和局部不变式的形式来评估双量子比特变换的特性。结果表明,在选择合适的管理参数值(如两个 QND 相互作用的持续时间和量子比特的旋转角度)时,该协议可以实现确定性非局部 SWAP 操作和纠缠 SWAP 操作,概率为 13。
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引用次数: 0
Separation of various higher-order effects in the ionization of helium by proton impact 质子撞击氦电离中各种高阶效应的分离
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-18 DOI: 10.1103/physreva.110.032814
S. Majumdar, S. Bastola, A. Hasan, R. Lomsadze, M. Schulz
We have measured fully differential cross sections (FDCSs) for ionization of helium by 75 keV proton impact. Data were analyzed for electrons ejected into the scattering plane at projectile energy losses well below and above the matching velocity and for scattering angles ranging between 0.1 and 0.5 mrad. Earlier, we observed clear signatures of the postcollision interaction (PCI) at the matching velocity; however, in the current data these signatures are completely absent at small energy losses and residues remain at large energy losses. At small energy losses the FDCSs are dominated by non-PCI higher-order effects.
我们测量了 75 keV 质子撞击氦电离的全差分截面 (FDCS)。我们分析了在射弹能量损失远低于和高于匹配速度以及散射角在 0.1 至 0.5 mrad 之间时射入散射平面的电子数据。早些时候,我们观察到碰撞后相互作用(PCI)在匹配速度下的明显特征;然而,在目前的数据中,这些特征在能量损失较小时完全消失,而在能量损失较大时仍有残留。在能量损失较小的情况下,非 PCI 高阶效应主导了 FDCS。
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引用次数: 0
Demonstration of superior communication through thermodynamically free channels in an optical quantum switch 通过光量子开关中的热力学自由通道演示卓越通信
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-18 DOI: 10.1103/physreva.110.032422
Hao Tang, Yu Guo, Xiao-Min Hu, Yun-Feng Huang, Bi-Heng Liu, Chuan-Feng Li, Guang-Can Guo
The release of the causal structure of physical events from a well-defined order to an indefinite order stimulates remarkable enhancements in various quantum information tasks. Some of these advantages, however, are questioned for the ambiguous role of the control system in the quantum switch, which is an experimentally realized process with an indefinite causal structure. In communications, for example, not only the superposition of alternative causal orders, but also the superposition of alternative trajectories can accelerate information transmissions. Here, we follow the proposal of Liu et al. [Phys. Rev. Lett. 129, 230604 (2022)], and examine the information enhancement effect of indefinite causal orders with the toolkit of thermodynamics in a photonic platform. Specifically, we simulate the thermal interaction between a system qubit and two heat baths embedded in a quantum switch by implementing the corresponding switched thermal channels. Although its action on the system qubit only is thermally free, our results suggest that the quantum switch should be seen as a resource when the control qubit is also considered. Moreover, we characterize the non-Markovian property in this scenario by measuring the information backflows from the heat baths to the system qubit.
物理事件的因果结构从定义明确的顺序变为不确定的顺序,激发了各种量子信息任务的显著提升。然而,由于量子开关中控制系统的作用不明确,其中一些优势受到质疑,因为量子开关是一个实验实现的过程,具有不确定的因果结构。例如,在通信中,不仅替代因果顺序的叠加,而且替代轨迹的叠加都能加速信息传输。在此,我们按照刘等人的建议[Phys. Rev. Lett. 129, 230604 (2022)],在光子平台上利用热力学工具包研究了不定因果顺序的信息增强效应。具体来说,我们通过实现相应的开关热通道,模拟了系统量子比特与嵌入量子开关的两个热浴之间的热相互作用。虽然量子开关对系统量子比特的作用是热自由的,但我们的结果表明,当同时考虑控制量子比特时,量子开关应被视为一种资源。此外,我们还通过测量从热浴到系统量子位的信息回流,描述了这种情况下的非马尔可夫特性。
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引用次数: 0
Probing the position-dependent optical energy fluence rate in three-dimensional scattering samples 探测三维散射样品中与位置相关的光能通量率
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-18 DOI: 10.1103/physreva.110.033520
Ozan Akdemir, Minh Duy Truong, Alfredo Rates, Ad Lagendijk, Willem L. Vos
The accurate determination of the position-dependent energy fluence rate of scattered light (which is proportional to the energy density) is crucial to the understanding of transport in anisotropically scattering and absorbing samples, such as biological tissue, seawater, atmospheric turbulent layers, and light-emitting diodes. While Monte Carlo simulations are precise, their long computation time is not desirable. Common analytical approximations to the radiative transfer equation (RTE) fail to predict light transport and could even give unphysical results. Therefore, we experimentally probe the position-dependent energy fluence rate of light inside scattering samples where the widely used P1 and P3 approximations to the RTE fail. The samples are three-dimensional (3D) aqueous suspensions of anisotropically scattering and both absorbing and nonabsorbing spherical scatterers, namely, microspheres (r=0.5µm) with and without absorbing dye. To probe the energy fluence rate, we detect the emission of quantum-dot reporter particles that are excited by the incident light and that are contained in a thin capillary. By scanning the capillary through the sample, we access the position dependence. We present a comprehensive discussion of experimental limitations and of both random and systematic errors. Our observations agree well with the Monte Carlo simulations and the P3 approximation of the RTE with a correction for forward scattering. In contrast, the P1 and the P3 approximations deviate increasingly from our observations, ultimately even predicting unphysical negative energies.
准确测定散射光随位置变化的能量通量率(与能量密度成正比),对于理解各向异性散射和吸收样品(如生物组织、海水、大气湍流层和发光二极管)中的传输至关重要。蒙特卡罗模拟虽然精确,但计算时间长,并不可取。辐射传递方程(RTE)的常见分析近似值无法预测光传输,甚至可能给出非物理结果。因此,我们通过实验探究了散射样品内光的位置依赖性能量通量率,在这些样品中,广泛使用的 P1 和 P3 近似 RTE 均失效。样品是由各向异性散射和吸收与非吸收球形散射体组成的三维(3D)水悬浮液,即含有和不含吸收染料的微球(r=0.5µm)。为了探测能量通量率,我们检测了被入射光激发并包含在细毛细管中的量子点报告粒子的发射。通过扫描穿过样品的毛细管,我们获得了位置依赖性。我们对实验限制以及随机误差和系统误差进行了全面讨论。我们的观测结果与蒙特卡罗模拟和修正了前向散射的 P3 近似 RTE 非常吻合。相比之下,P1 和 P3 近似值与我们的观测结果偏差越来越大,最终甚至预测出了非物理的负能量。
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引用次数: 0
Fundamental constants from photon-photon scattering in three-beam collisions 三光束碰撞中光子-光子散射的基本常数
IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Pub Date : 2024-09-18 DOI: 10.1103/physreva.110.032216
A. J. MacLeod, B. King
Direct measurement of the elastic scattering of real photons on an electromagnetic field would allow the fundamental low-energy constants of quantum electrodynamics to be experimentally determined. We show that scenarios involving the collision of three laser beams have several advantages over conventional two-beam scenarios. The kinematics of a three-beam collision allows for a higher signal-to-background ratio in the detection region, without the need for polarimetry, and separates out contributions from different orders of photon scattering. A planar configuration of colliding a photon beam from an x-ray free-electron laser with two optical beams is studied in detail. We show that measurements of elastic photon scattering and vacuum birefringence are possible with currently available technology.
直接测量真实光子在电磁场上的弹性散射,可以通过实验确定量子电动力学的基本低能常数。我们的研究表明,与传统的双光束方案相比,涉及三束激光碰撞的方案具有若干优势。三光束碰撞的运动学原理使探测区域的信噪比更高,无需偏振测量法,并能分离出不同数量级的光子散射。我们详细研究了将来自 X 射线自由电子激光器的光子束与两束光束碰撞的平面配置。我们表明,利用现有技术可以测量弹性光子散射和真空双折射。
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引用次数: 0
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Physical Review A
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