Nanoscale zero-valent iron composites for uranium-contaminated water treatment and environmental remediation: A review

IF 8.3 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2024-09-24 DOI:10.1039/d4en00613e
Yinshan Zhu, Shusen Chen, Ziming Li, Hao Li, Muhammad Shaban, Changlun Chen
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Abstract

With the development of nuclear power and the nuclear industry, some uranium-containing wastewater will inevitably be released into the environment, which poses a threat to human health and the environment. Nanoscale zero-valent iron (nZVI) and its composites can be used to treat uranium-contaminated water because of its large specific surface area, many active centres and high adsorption capacity. This review proposed a matrix loaded zero-valent iron, including bimetals, inorganic materials, carbon materials, and organic and porous framework materials. The latest research progress of various nZVI-based composites in removing uranium from aqueous solutions was reviewed. A detailed introduction to the preparation methods, removal mechanisms, and environmental factors affecting the removal performance of nZVI and its composite materials was provided. The advantages and disadvantages of nZVI and its composite materials for uranium removal were analyzed, and loading methods conducive to solving the dispersion and agglomeration problems of nZVI were emphasized. Finally, the application prospects of nZVI and its composites in the remediation of uranium-contaminated water were briefly proposed, and the application prospects in environmental remediation were discussed.
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用于铀污染水处理和环境修复的纳米级零价铁复合材料:综述
随着核电和核工业的发展,一些含铀废水不可避免地会排放到环境中,对人类健康和环境造成威胁。纳米级零价铁(nZVI)及其复合材料具有比表面积大、活性中心多、吸附能力强等特点,可用于处理铀污染水。本综述提出了负载零价铁的基质,包括双金属、无机材料、碳材料以及有机和多孔框架材料。综述了各种基于 nZVI 的复合材料从水溶液中去除铀的最新研究进展。详细介绍了 nZVI 及其复合材料的制备方法、去除机理以及影响去除性能的环境因素。分析了 nZVI 及其复合材料在脱铀方面的优缺点,强调了有利于解决 nZVI 分散和团聚问题的负载方法。最后,简要提出了 nZVI 及其复合材料在铀污染水体修复中的应用前景,并讨论了其在环境修复中的应用前景。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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